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231225s2022 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202103963
|2 doi
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|a pubmed24n1107.xml
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|a (DE-627)NLM332126056
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|a (NLM)34672402
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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|a Lamaison, Sarah
|e verfasserin
|4 aut
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|a Designing a Zn-Ag Catalyst Matrix and Electrolyzer System for CO2 Conversion to CO and Beyond
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|c 2022
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Revised 07.01.2022
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2021 Wiley-VCH GmbH.
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|a CO2 emissions can be transformed into high-added-value commodities through CO2 electrocatalysis; however, efficient low-cost electrocatalysts are needed for global scale-up. Inspired by other emerging technologies, the authors report the development of a gas diffusion electrode containing highly dispersed Ag sites in a low-cost Zn matrix. This catalyst shows unprecedented Ag mass activity for CO production: -614 mA cm-2 at 0.17 mg of Ag. Subsequent electrolyte engineering demonstrates that halide anions can further improve stability and activity of the Zn-Ag catalyst, outperforming pure Ag and Au. Membrane electrode assemblies are constructed and coupled to a microbial process that converts the CO to acetate and ethanol. Combined, these concepts present pathways to design catalysts and systems for CO2 conversion toward sought-after products
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|a Journal Article
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|a carbon dioxide conversion
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|a carbon monoxide
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|a gas diffusion electrodes
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|a mass activities
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|a membrane electrode assemblies
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|a microbial coupling
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|a multiphysics models
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|a Wakerley, David
|e verfasserin
|4 aut
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|a Kracke, Frauke
|e verfasserin
|4 aut
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|a Moore, Thomas
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|a Zhou, Lan
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|a Lee, Dong Un
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|a Wang, Lei
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|a Hubert, McKenzie A
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|a Aviles Acosta, Jaime E
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|4 aut
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|a Gregoire, John M
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|4 aut
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|a Duoss, Eric B
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|4 aut
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|a Baker, Sarah
|e verfasserin
|4 aut
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|a Beck, Victor A
|e verfasserin
|4 aut
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|a Spormann, Alfred M
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|4 aut
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|a Fontecave, Marc
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|4 aut
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|a Hahn, Christopher
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|4 aut
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|a Jaramillo, Thomas F
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 34(2022), 1 vom: 19. Jan., Seite e2103963
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:34
|g year:2022
|g number:1
|g day:19
|g month:01
|g pages:e2103963
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|u http://dx.doi.org/10.1002/adma.202103963
|3 Volltext
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