Hierarchically Structured P-Doped MoS2/MoO2 Ultrathin Nanosheets on N-Doped Carbon Hemispheres for Sensitive Dopamine Detection

Dopamine (DA) is a key neurotransmitter in the central nervous system, and abnormal concentrations are associated with a variety of diseases. In this study, a novel electrochemical sensor is constructed based on ultrathin P-doped MoS2/MoO2 nanosheets supported on bowl-shaped N-doped carbon hemispher...

Ausführliche Beschreibung

Bibliographische Detailangaben
Veröffentlicht in:Langmuir : the ACS journal of surfaces and colloids. - 1985. - 41(2025), 31 vom: 12. Aug., Seite 20723-20733
1. Verfasser: Xu, Li (VerfasserIn)
Weitere Verfasser: Hu, Pingyue, Tan, Liwen, Guo, Junchun, Li, Sheng, Xiong, Xiaoli
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2025
Zugriff auf das übergeordnete Werk:Langmuir : the ACS journal of surfaces and colloids
Schlagworte:Journal Article Molybdenum 81AH48963U Dopamine VTD58H1Z2X Disulfides molybdenum disulfide ZC8B4P503V Carbon 7440-44-0 mehr... Oxides molybdenum dioxide
LEADER 01000caa a22002652c 4500
001 NLM390227668
003 DE-627
005 20250812232146.0
007 cr uuu---uuuuu
008 250730s2025 xx |||||o 00| ||eng c
024 7 |a 10.1021/acs.langmuir.5c02156  |2 doi 
028 5 2 |a pubmed25n1528.xml 
035 |a (DE-627)NLM390227668 
035 |a (NLM)40735867 
040 |a DE-627  |b ger  |c DE-627  |e rakwb 
041 |a eng 
100 1 |a Xu, Li  |e verfasserin  |4 aut 
245 1 0 |a Hierarchically Structured P-Doped MoS2/MoO2 Ultrathin Nanosheets on N-Doped Carbon Hemispheres for Sensitive Dopamine Detection 
264 1 |c 2025 
336 |a Text  |b txt  |2 rdacontent 
337 |a ƒaComputermedien  |b c  |2 rdamedia 
338 |a ƒa Online-Ressource  |b cr  |2 rdacarrier 
500 |a Date Completed 12.08.2025 
500 |a Date Revised 12.08.2025 
500 |a published: Print-Electronic 
500 |a Citation Status MEDLINE 
520 |a Dopamine (DA) is a key neurotransmitter in the central nervous system, and abnormal concentrations are associated with a variety of diseases. In this study, a novel electrochemical sensor is constructed based on ultrathin P-doped MoS2/MoO2 nanosheets supported on bowl-shaped N-doped carbon hemispheres (N-BCHP-MoS2/MoO2). The unique hierarchical structure combines the high specific surface area of N-BCH with the enhanced electrocatalytic activity of P-doped MoS2/MoO2, resulting in significant improvements in the performance for DA detection. The electronic structure of the catalyst is further modulated by the codoping of N and P, which increases the electrical conductivity and the number of active centers. The results show that the N-BCH@P-MoS2/MoO2 exhibits excellent sensitivity and selectivity for DA detection, capable of achieving a detection limit as low as 0.12 μM within a broad concentration range (3-100 μM) (S/N = 3). Furthermore, electrocatalysts have been employed in the detection of DA in human serum, indicating significant promise for clinical diagnosis 
650 4 |a Journal Article 
650 7 |a Molybdenum  |2 NLM 
650 7 |a 81AH48963U  |2 NLM 
650 7 |a Dopamine  |2 NLM 
650 7 |a VTD58H1Z2X  |2 NLM 
650 7 |a Disulfides  |2 NLM 
650 7 |a molybdenum disulfide  |2 NLM 
650 7 |a ZC8B4P503V  |2 NLM 
650 7 |a Carbon  |2 NLM 
650 7 |a 7440-44-0  |2 NLM 
650 7 |a Oxides  |2 NLM 
650 7 |a molybdenum dioxide  |2 NLM 
700 1 |a Hu, Pingyue  |e verfasserin  |4 aut 
700 1 |a Tan, Liwen  |e verfasserin  |4 aut 
700 1 |a Guo, Junchun  |e verfasserin  |4 aut 
700 1 |a Li, Sheng  |e verfasserin  |4 aut 
700 1 |a Xiong, Xiaoli  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Langmuir : the ACS journal of surfaces and colloids  |d 1985  |g 41(2025), 31 vom: 12. Aug., Seite 20723-20733  |w (DE-627)NLM098181009  |x 1520-5827  |7 nnas 
773 1 8 |g volume:41  |g year:2025  |g number:31  |g day:12  |g month:08  |g pages:20723-20733 
856 4 0 |u http://dx.doi.org/10.1021/acs.langmuir.5c02156  |3 Volltext 
912 |a GBV_USEFLAG_A 
912 |a SYSFLAG_A 
912 |a GBV_NLM 
912 |a GBV_ILN_22 
912 |a GBV_ILN_350 
912 |a GBV_ILN_721 
951 |a AR 
952 |d 41  |j 2025  |e 31  |b 12  |c 08  |h 20723-20733