Pretreatment for potable reuse : Enhancing the biological removal of 1,4-dioxane from landfill leachate through cometabolism with tetrahydrofuran
© 2024 The Author(s). Water Environment Research published by Wiley Periodicals LLC on behalf of Water Environment Federation.
Veröffentlicht in: | Water environment research : a research publication of the Water Environment Federation. - 1998. - 96(2024), 8 vom: 15. Aug., Seite e11108 |
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Weitere Verfasser: | , , , , , |
Format: | Online-Aufsatz |
Sprache: | English |
Veröffentlicht: |
2024
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Zugriff auf das übergeordnete Werk: | Water environment research : a research publication of the Water Environment Federation |
Schlagworte: | Journal Article 1,4‐dioxane leachate moving bed biofilm reactor potable reuse tetrahydrofuran Dioxanes 1,4-dioxane J8A3S10O7S Water Pollutants, Chemical mehr... |
Zusammenfassung: | © 2024 The Author(s). Water Environment Research published by Wiley Periodicals LLC on behalf of Water Environment Federation. 1,4-Dioxane is a probable human carcinogen and a persistent aquatic contaminant. Cometabolic biodegradation of 1,4-dioxane is a promising low-cost and effective treatment technology; however, further demonstration is needed for treating landfill leachate. This technology was tested in two full-scale moving bed biofilm reactors (MBBRs) treating raw landfill leachate with tetrahydrofuran selected as the cometabolite. The raw leachate contained on average 82 μg/L of 1,4-dioxane and before testing the MBBRs removed an average of 38% and 42% of 1,4-dioxane, respectively. First, tetrahydrofuran was added to MBBR 1, and 1,4-dioxane removal was improved to an average of 73%, with the control MBBR removing an average of 37% of 1,4-dioxane. During this period, an optimal dose of 2 mg/L of tetrahydrofuran was identified. Tetrahydrofuran was then fed to both MBBRs, where the 1,4-dioxane removal was on average 73% and 80%. Cometabolic treatment at the landfill significantly reduced the concentration of 1,4-dioxane received from the landfill at a downstream wastewater treatment and indirect potable reuse facility, reducing the load of 1,4-dioxane from 44% to 24% after the study. PRACTITIONER POINTS: Cometabolic degradation of leachate 1,4-dioxane with THF in MBBRs is a feasible treatment technology and a low-cost technique when retrofitting existing biological treatment facilities. The MBBRs can be operated at a range of temperatures, require no operational changes beyond THF addition, and operate best at a mass ratio of THF to 1,4-dioxane of 24. Source control of 1,4-dioxane significantly reduces the concentration of 1,4-dioxane in downstream wastewater treatment plants and potable reuse facilities |
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Beschreibung: | Date Completed 15.08.2024 Date Revised 15.08.2024 published: Print Citation Status MEDLINE |
ISSN: | 1554-7531 |
DOI: | 10.1002/wer.11108 |