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240404s2024 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202401858
|2 doi
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|a pubmed24n1474.xml
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|a eng
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1 |
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|a Dou, Haozhen
|e verfasserin
|4 aut
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1 |
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|a Biomass Solid-State Electrolyte with Abundant Ion and Water Channels for Flexible Zinc-Air Batteries
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|c 2024
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|a Text
|b txt
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|a ƒaComputermedien
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|a ƒa Online-Ressource
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|a Date Revised 18.07.2024
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2024 Wiley‐VCH GmbH.
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|a Flexible zinc-air batteries are the leading candidates as the next-generation power source for flexible/wearable electronics. However, constructing safe and high-performance solid-state electrolytes (SSEs) with intrinsic hydroxide ion (OH-) conduction remains a fundamental challenge. Herein, by adopting the natural and robust cellulose nanofibers (CNFs) as building blocks, the biomass SSEs with penetrating ion and water channels are constructed by knitting the OH--conductive CNFs and water-retentive CNFs together via an energy-efficient tape casting. Benefiting from the abundant ion and water channels with interconnected hydrated OH- wires for fast OH- conduction under a nanoconfined environment, the biomass SSEs reveal the high water-uptake, impressive OH- conductivity of 175 mS cm-1 and mechanical robustness simultaneously, which overcomes the commonly existed dilemma between ion conductivity and mechanical property. Remarkably, the flexible zinc-air batteries assemble with biomass SSEs deliver an exceptional cycle lifespan of 310 h and power density of 126 mW cm-2. The design methodology for water and ion channels opens a new avenue to design high-performance SSEs for batteries
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|a Journal Article
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|a cellulose nanofibers
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| 650 |
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4 |
|a flexible zinc–air batteries
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| 650 |
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4 |
|a ion channels
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| 650 |
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4 |
|a solid‐state electrolytes
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| 650 |
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4 |
|a water channels
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| 700 |
1 |
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|a Xu, Mi
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Zhang, Zhen
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Luo, Dan
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Yu, Aiping
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Chen, Zhongwei
|e verfasserin
|4 aut
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| 773 |
0 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 29 vom: 23. Juli, Seite e2401858
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:36
|g year:2024
|g number:29
|g day:23
|g month:07
|g pages:e2401858
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| 856 |
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|u http://dx.doi.org/10.1002/adma.202401858
|3 Volltext
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