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240125s2024 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202311305
|2 doi
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|a pubmed24n1395.xml
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|a (DE-627)NLM36760714X
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|a (NLM)38270280
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|a DE-627
|b ger
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|a eng
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| 100 |
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|a Xu, Tao
|e verfasserin
|4 aut
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|a Boosting the Performances of Semitransparent Organic Photovoltaics via Synergetic Near-Infrared Light Management
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|c 2024
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|a Text
|b txt
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Revised 02.05.2024
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2024 Wiley‐VCH GmbH.
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|a Semitransparent organic photovoltaics (ST-OPVs) offer promising prospects for application in building-integrated photovoltaic systems and greenhouses, but further improvement of their performance faces a delicate trade-off between the two competing indexes of power conversion efficiency (PCE) and average visible transmittance (AVT). Herein, the authors take advantage of coupling plasmonics with the optical design of ST-OPVs to enhance near-infrared absorption and hence simultaneously improve efficiency and visible transparency to the maximum extent. By integrating core-bishell PdCuAu@SiO2 nanotripods that act as optically isotropic Lambertian sources with near-infrared-customized localized surface plasmon resonance in an optimal ternary PM6:BTP-eC9:L8-BO-based ST-OPV, it is shown that their interplay with a multilayer optical coupling layer, consisting of ZnS(130 nm)/Na3AlF6(60 nm)/WO3(100 nm)/LaF3(50 nm) identified from high-throughput optical screening, leads to a record-high PCE of 16.14% (certified as 15.90%) along with an excellent AVT of 33.02%. The strong enhancement of the light utilization efficiency by ≈50% as compared to the counterpart device without optical engineering provides an encouraging and universal pathway for promoting breakthroughs in ST-OPVs from meticulous optical design
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|a Journal Article
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|a high‐throughput optical screening
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|a near‐infrared absorption enhancement
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|a optical engineering
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|a plasmonics
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|a semitransparent organic photovoltaics
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|a Deng, Baozhong
|e verfasserin
|4 aut
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|a Zheng, Kaiwen
|e verfasserin
|4 aut
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|a Li, Hongyu
|e verfasserin
|4 aut
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|a Wang, Zihan
|e verfasserin
|4 aut
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|a Zhong, Yunbo
|e verfasserin
|4 aut
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| 700 |
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|a Zhang, Chengxi
|e verfasserin
|4 aut
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|a Lévêque, Gaëtan
|e verfasserin
|4 aut
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|a Grandidier, Bruno
|e verfasserin
|4 aut
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|a Bachelot, Renaud
|e verfasserin
|4 aut
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|a Treguer-Delapierre, Mona
|e verfasserin
|4 aut
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|a Qi, Yabing
|e verfasserin
|4 aut
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| 700 |
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|a Wang, Shenghao
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 18 vom: 01. Mai, Seite e2311305
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:36
|g year:2024
|g number:18
|g day:01
|g month:05
|g pages:e2311305
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|u http://dx.doi.org/10.1002/adma.202311305
|3 Volltext
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