Enhanced dewatering extent of sludge by Fe3O4-driven heterogeneous Fenton

Copyright © 2023 Elsevier Ltd. All rights reserved.

Bibliographische Detailangaben
Veröffentlicht in:Waste management (New York, N.Y.). - 1999. - 174(2024) vom: 15. Jan., Seite 666-673
1. Verfasser: Li, Ting (VerfasserIn)
Weitere Verfasser: Zhang, Xin, Zhou, Yujun, Yang, Jiawei, Cheng, Fange, Fang, Di, Liang, Jianru, Li, Jiansheng, Zhou, Lixiang
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2024
Zugriff auf das übergeordnete Werk:Waste management (New York, N.Y.)
Schlagworte:Journal Article Fe(3)O(4) Heterogeneous Fenton Improvement mechanism Sludge dewatering Sewage Hydrogen Peroxide BBX060AN9V Iron E1UOL152H7 mehr... Water 059QF0KO0R
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245 1 0 |a Enhanced dewatering extent of sludge by Fe3O4-driven heterogeneous Fenton 
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520 |a Homogeneous Fenton (Fe2+/H2O2) serves as a high-efficiency conditioning method for sludge dewatering due to the generation of strong oxidizing hydroxyl radicals (OH). However, high dose of ferric salts produces iron-rich dewatered sludge and decrease sludge organic matters, which will not be conducive to the subsequent disposal and reutilization. Considering advantages of Fe3O4 as heterogeneous Fenton catalyst, Fe3O4-activated H2O2 (Fe3O4 + H2O2) in this study was adopted to improve sludge deep-dewatering. Reduction efficiency of the bound water (71.3 %) after Fe3O4 + H2O2 treatment (after a reaction time of 30 min) were much higher than those in the Fe2++H2O2 treatment. Especially, the moisture content of treated sludge cake by Fe3O4 + H2O2 remarkably decreased from 86.4 % to 61.3 %. Improvement mechanism of sludge dewatering after Fe3O4 + H2O2 treatment mainly included electrostatic neutralization, reactive radical oxidation, and skeleton building by analysis of contribution factors. The generation of H+ in acidification could neutralize the negatively charged compounds to promote sludge hydrophobicity. Meanwhile reactive radicals generated from Fe3O4 + H2O2 destroyed sludge extracellular polymeric substances and cell structure to release intracellular water. Furthermore, Fe3O4 as a skeleton builder could reconstruct destructive sludge flocs and form new dewatering channels. Finally, low Fe leaching content and recoverability of Fe3O4 effectively will decrease environmental implication 
650 4 |a Journal Article 
650 4 |a Fe(3)O(4) 
650 4 |a Heterogeneous Fenton 
650 4 |a Improvement mechanism 
650 4 |a Sludge dewatering 
650 7 |a Sewage  |2 NLM 
650 7 |a Hydrogen Peroxide  |2 NLM 
650 7 |a BBX060AN9V  |2 NLM 
650 7 |a Iron  |2 NLM 
650 7 |a E1UOL152H7  |2 NLM 
650 7 |a Water  |2 NLM 
650 7 |a 059QF0KO0R  |2 NLM 
700 1 |a Zhang, Xin  |e verfasserin  |4 aut 
700 1 |a Zhou, Yujun  |e verfasserin  |4 aut 
700 1 |a Yang, Jiawei  |e verfasserin  |4 aut 
700 1 |a Cheng, Fange  |e verfasserin  |4 aut 
700 1 |a Fang, Di  |e verfasserin  |4 aut 
700 1 |a Liang, Jianru  |e verfasserin  |4 aut 
700 1 |a Li, Jiansheng  |e verfasserin  |4 aut 
700 1 |a Zhou, Lixiang  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Waste management (New York, N.Y.)  |d 1999  |g 174(2024) vom: 15. Jan., Seite 666-673  |w (DE-627)NLM098197061  |x 1879-2456  |7 nnns 
773 1 8 |g volume:174  |g year:2024  |g day:15  |g month:01  |g pages:666-673 
856 4 0 |u http://dx.doi.org/10.1016/j.wasman.2023.12.044  |3 Volltext 
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