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231226s2024 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202307298
|2 doi
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|a eng
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| 100 |
1 |
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|a Zhang, Xinyuan
|e verfasserin
|4 aut
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| 245 |
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|a High-Sulfur Loading and Single Ion-Selective Membranes for High-Energy and Durable Decoupled Aqueous Batteries
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|c 2024
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|a Text
|b txt
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Revised 18.01.2024
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2023 Wiley-VCH GmbH.
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|a The decoupled battery design is promising for breaking the energy density limit of traditional aqueous batteries. However, the complex battery configuration and low-selective separator membranes restrict their energy output and service time. Herein, a zinc-sulfur decoupled aqueous battery is achieved by designing a high-mass loading sulfur electrode and single ion-selective membrane (ISM). A vertically assembled nanosheet network constructed with the assistance of a magnetic field enables facile electron and ion conduction in thick sulfur electrodes, which is conducive to boosting the cell-level energy output. For the tailored ISM, the Na ions anchored on its skeleton effectively prevent the crossover of OH- or Cu2+ , facilitating the transport of Na+ and ensuring structural and mechanical stability. Consequently, the Zn-S aqueous battery achieves a reversible energy density of 3988 Wh kgs -1 (by sulfur mass), stable operation over 300 cycles, and an energy density of 53.2 mWh cm-2 . The sulfur-based decoupled system may be of immediate benefit toward safe, reliable, and affordable static energy storage
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|a Journal Article
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|a Zn-S aqueous batteries
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|a decoupled batteries
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|a high sulfur loading
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|a ion channels
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| 650 |
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|a ion-selective membranes
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| 700 |
1 |
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|a Zhang, Bao
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Yang, Jin-Lin
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Wu, Jiawen
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Jiang, Heng
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Du, Fei
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Fan, Hong Jin
|e verfasserin
|4 aut
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| 773 |
0 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 3 vom: 01. Jan., Seite e2307298
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:36
|g year:2024
|g number:3
|g day:01
|g month:01
|g pages:e2307298
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|u http://dx.doi.org/10.1002/adma.202307298
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