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231226s2023 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202203547
|2 doi
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|a pubmed24n1171.xml
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|a (DE-627)NLM351607919
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|a (NLM)36649977
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|a DE-627
|b ger
|c DE-627
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|a eng
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|a Li, Xinle
|e verfasserin
|4 aut
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|a An Ultrathin Nonporous Polymer Separator Regulates Na Transfer Toward Dendrite-Free Sodium Storage Batteries
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|c 2023
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Completed 13.04.2023
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|a Date Revised 13.04.2023
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2023 Wiley-VCH GmbH.
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|a Sodium storage batteries are one of the ever-increasing next-generation large-scale energy storage systems owing to the abundant resources and low cost. However, their viability is severely hampered by dendrite-related hazards on anodes. Herein, a novel ultrathin (8 µm) exterior-nonporous separator composed of honeycomb-structured fibers is prepared for homogeneous Na deposition and suppressed dendrite penetration. The unhindered ion transmission greatly benefits from honeycomb-structured fibers with huge electrolyte uptake (376.7%) and the polymer's inherent transport ability. Additionally, polar polymer chains consisting of polyethersulfone and polyvinylidene customize the highly aggregated solvation structure of electrolytes via substantial solvent immobilization, facilitating ion-conductivity-enhanced inorganic-rich solid-electrolyte interphase with remarkable interface endurance. With the reliable mechanical strength of the separator, the assembled sodium-ion full cell delivers significantly improved energy density and high safety, enabling stable operation under cutting and rolling. The as-prepared separator can further be generalized to lithium-based batteries for which apparent dendrite inhibition and cyclability are accessible and demonstrates its potential for practical application
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|a Journal Article
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|a dendrite
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|a high-energy density
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|a high-safety
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|a separator
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|a sodium-ion batteries
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|a Zhang, Jiyu
|e verfasserin
|4 aut
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|a Guo, Xiaoniu
|e verfasserin
|4 aut
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|a Peng, Chengbin
|e verfasserin
|4 aut
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|a Song, Keming
|e verfasserin
|4 aut
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|a Zhang, Zhiguo
|e verfasserin
|4 aut
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|a Ding, Lina
|e verfasserin
|4 aut
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|a Liu, Chuntai
|e verfasserin
|4 aut
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|a Chen, Weihua
|e verfasserin
|4 aut
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|a Dou, Shixue
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 35(2023), 15 vom: 17. Apr., Seite e2203547
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:35
|g year:2023
|g number:15
|g day:17
|g month:04
|g pages:e2203547
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|u http://dx.doi.org/10.1002/adma.202203547
|3 Volltext
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