|
|
|
|
| LEADER |
01000naa a22002652 4500 |
| 001 |
NLM332814254 |
| 003 |
DE-627 |
| 005 |
20231225220343.0 |
| 007 |
cr uuu---uuuuu |
| 008 |
231225s2022 xx |||||o 00| ||eng c |
| 024 |
7 |
|
|a 10.1002/adma.202107104
|2 doi
|
| 028 |
5 |
2 |
|a pubmed24n1109.xml
|
| 035 |
|
|
|a (DE-627)NLM332814254
|
| 035 |
|
|
|a (NLM)34743375
|
| 040 |
|
|
|a DE-627
|b ger
|c DE-627
|e rakwb
|
| 041 |
|
|
|a eng
|
| 100 |
1 |
|
|a Wang, Yadong
|e verfasserin
|4 aut
|
| 245 |
1 |
0 |
|a Probing Electronic States in Monolayer Semiconductors through Static and Transient Third-Harmonic Spectroscopies
|
| 264 |
|
1 |
|c 2022
|
| 336 |
|
|
|a Text
|b txt
|2 rdacontent
|
| 337 |
|
|
|a ƒaComputermedien
|b c
|2 rdamedia
|
| 338 |
|
|
|a ƒa Online-Ressource
|b cr
|2 rdacarrier
|
| 500 |
|
|
|a Date Revised 21.01.2022
|
| 500 |
|
|
|a published: Print-Electronic
|
| 500 |
|
|
|a Citation Status PubMed-not-MEDLINE
|
| 520 |
|
|
|a © 2021 Wiley-VCH GmbH.
|
| 520 |
|
|
|a Electronic states and their dynamics are of critical importance for electronic and optoelectronic applications. Here, various relevant electronic states in monolayer MoS2 , such as multiple excitonic Rydberg states and free-particle energy bands are probed with a high relative contrast of up to ≥200 via broadband (from ≈1.79 to 3.10 eV) static third-harmonic spectroscopy (THS), which is further supported by theoretical calculations. Moreover, transient THS is introduced to demonstrate that third-harmonic generation can be all-optically modulated with a modulation depth exceeding ≈94% at ≈2.18 eV, providing direct evidence of dominant carrier relaxation processes associated with carrier-exciton and carrier-phonon interactions. The results indicate that static and transient THS are not only promising techniques for the characterization of monolayer semiconductors and their heterostructures, but also a potential platform for disruptive photonic and optoelectronic applications, including all-optical modulation and imaging
|
| 650 |
|
4 |
|a Journal Article
|
| 650 |
|
4 |
|a electronic states
|
| 650 |
|
4 |
|a monolayer transition metal dichalcogenides
|
| 650 |
|
4 |
|a static third-harmonic spectroscopy
|
| 650 |
|
4 |
|a third-harmonic generation
|
| 650 |
|
4 |
|a transient third-harmonic spectroscopy
|
| 700 |
1 |
|
|a Iyikanat, Fadil
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Rostami, Habib
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Bai, Xueyin
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Hu, Xuerong
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Das, Susobhan
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Dai, Yunyun
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Du, Luojun
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Zhang, Yi
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Li, Shisheng
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Lipsanen, Harri
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a García de Abajo, F Javier
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Sun, Zhipei
|e verfasserin
|4 aut
|
| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 34(2022), 3 vom: 06. Jan., Seite e2107104
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
|
| 773 |
1 |
8 |
|g volume:34
|g year:2022
|g number:3
|g day:06
|g month:01
|g pages:e2107104
|
| 856 |
4 |
0 |
|u http://dx.doi.org/10.1002/adma.202107104
|3 Volltext
|
| 912 |
|
|
|a GBV_USEFLAG_A
|
| 912 |
|
|
|a SYSFLAG_A
|
| 912 |
|
|
|a GBV_NLM
|
| 912 |
|
|
|a GBV_ILN_350
|
| 951 |
|
|
|a AR
|
| 952 |
|
|
|d 34
|j 2022
|e 3
|b 06
|c 01
|h e2107104
|