Large Switchable Photoconduction within 2D Potential Well of a Layered Ferroelectric Heterostructure

© 2020 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 32(2020), 37 vom: 23. Sept., Seite e2003033
1. Verfasser: Yang, Yuben (VerfasserIn)
Weitere Verfasser: Mao, Huican, Wang, Jing, Zhang, Qinghua, Jin, Lei, Wang, Chuanshou, Zhang, Yuelin, Su, Nan, Meng, Fanqi, Yang, Ying, Xia, Ruqiao, Chen, Rongyan, Zhu, Hui, Gu, Lin, Yin, Zhiping, Nan, Ce-Wen, Zhang, Jinxing
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2020
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article 2D potential wells Bi2WO6 layered ferroelectric materials photovoltaics switchable photoconduction
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245 1 0 |a Large Switchable Photoconduction within 2D Potential Well of a Layered Ferroelectric Heterostructure 
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520 |a The coexistence of large conductivity and robust ferroelectricity is promising for high-performance ferroelectric devices based on polarization-controllable highly efficient carrier transport. Distinct from traditional perovskite ferroelectrics, Bi2 WO6 with a layered structure shows a great potential to preserve its ferroelectricity under substantial electron doping. Herein, by artificial design of photosensitive heterostructures with desired band alignment, three orders of magnitude enhancement of the short-circuit photocurrent is achieved in Bi2 WO6 /SrTiO3 at room temperature. The microscopic mechanism of this large photocurrent originates from separated transport of electrons and holes in [WO4 ]-2 and [Bi2 O2 ]+2 layers respectively with a large in-plane conductivity, which is understood by a combination of ab initio calculations and spectroscopic measurements. The layered electronic structure and appropriately designed band alignment in this layered ferroelectric heterostructure provide an opportunity to achieve high-performance and nonvolatile switchable electronic devices 
650 4 |a Journal Article 
650 4 |a 2D potential wells 
650 4 |a Bi2WO6 
650 4 |a layered ferroelectric materials 
650 4 |a photovoltaics 
650 4 |a switchable photoconduction 
700 1 |a Mao, Huican  |e verfasserin  |4 aut 
700 1 |a Wang, Jing  |e verfasserin  |4 aut 
700 1 |a Zhang, Qinghua  |e verfasserin  |4 aut 
700 1 |a Jin, Lei  |e verfasserin  |4 aut 
700 1 |a Wang, Chuanshou  |e verfasserin  |4 aut 
700 1 |a Zhang, Yuelin  |e verfasserin  |4 aut 
700 1 |a Su, Nan  |e verfasserin  |4 aut 
700 1 |a Meng, Fanqi  |e verfasserin  |4 aut 
700 1 |a Yang, Ying  |e verfasserin  |4 aut 
700 1 |a Xia, Ruqiao  |e verfasserin  |4 aut 
700 1 |a Chen, Rongyan  |e verfasserin  |4 aut 
700 1 |a Zhu, Hui  |e verfasserin  |4 aut 
700 1 |a Gu, Lin  |e verfasserin  |4 aut 
700 1 |a Yin, Zhiping  |e verfasserin  |4 aut 
700 1 |a Nan, Ce-Wen  |e verfasserin  |4 aut 
700 1 |a Zhang, Jinxing  |e verfasserin  |4 aut 
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773 1 8 |g volume:32  |g year:2020  |g number:37  |g day:23  |g month:09  |g pages:e2003033 
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