Origins of High Performance and Degradation in the Mixed Perovskite Solar Cells

© 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 31(2019), 8 vom: 15. Feb., Seite e1805438
1. Verfasser: Heo, Sung (VerfasserIn)
Weitere Verfasser: Seo, Gabseok, Lee, Yonghui, Seol, Minsu, Kim, Seong Heon, Yun, Dong-Jin, Kim, Yongsu, Kim, Kihong, Lee, Junho, Lee, Jooho, Jeon, Woo Sung, Shin, Jai Kwang, Park, Jucheol, Lee, Dongwook, Nazeeruddin, Mohammad Khaja
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2019
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article defect degradation long-term stability mixed perovskite perovskite solar cells
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520 |a The origins of the high device performance and degradation in the air are the greatest issues for commercialization of perovskite solar cells. Here this study investigates the possible origins of the mixed perovskite cells by monitoring defect states and compositional changes of the perovskite layer over the time. The results of deep-level transient spectroscopy analysis reveal that a newly identified defect formed by Br atoms exists at deep levels of the mixed perovskite film, and its defect state shifts when the film is aged in the air. The change of the defect state is originated from loss of the methylammonium molecules of the perovskite layer, which results in decreased JSC , deterioration of the power conversion efficiency and long-term stability of perovskite solar cells. The results provide a powerful strategy to diagnose and manage the efficiency and stability of perovskite solar cells 
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650 4 |a defect 
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650 4 |a long-term stability 
650 4 |a mixed perovskite 
650 4 |a perovskite solar cells 
700 1 |a Seo, Gabseok  |e verfasserin  |4 aut 
700 1 |a Lee, Yonghui  |e verfasserin  |4 aut 
700 1 |a Seol, Minsu  |e verfasserin  |4 aut 
700 1 |a Kim, Seong Heon  |e verfasserin  |4 aut 
700 1 |a Yun, Dong-Jin  |e verfasserin  |4 aut 
700 1 |a Kim, Yongsu  |e verfasserin  |4 aut 
700 1 |a Kim, Kihong  |e verfasserin  |4 aut 
700 1 |a Lee, Junho  |e verfasserin  |4 aut 
700 1 |a Lee, Jooho  |e verfasserin  |4 aut 
700 1 |a Jeon, Woo Sung  |e verfasserin  |4 aut 
700 1 |a Shin, Jai Kwang  |e verfasserin  |4 aut 
700 1 |a Park, Jucheol  |e verfasserin  |4 aut 
700 1 |a Lee, Dongwook  |e verfasserin  |4 aut 
700 1 |a Nazeeruddin, Mohammad Khaja  |e verfasserin  |4 aut 
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