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231225s2017 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201703028
|2 doi
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|a pubmed24n0923.xml
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|a (DE-627)NLM276930010
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|a (NLM)29024100
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|a DE-627
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|e rakwb
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|a eng
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| 100 |
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|a Liu, Yajie
|e verfasserin
|4 aut
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| 245 |
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|a An All-Integrated Anode via Interlinked Chemical Bonding between Double-Shelled-Yolk-Structured Silicon and Binder for Lithium-Ion Batteries
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|c 2017
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
|b cr
|2 rdacarrier
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|a Date Completed 18.07.2018
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|a Date Revised 01.10.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a The concept of an all-integrated design with multifunctionalization is widely employed in optoelectronic devices, sensors, resonator systems, and microfluidic devices, resulting in benefits for many ongoing research projects. Here, maintaining structural/electrode stability against large volume change by means of an all-integrated design is realized for silicon anodes. An all-integrated silicon anode is achieved via multicomponent interlinking among carbonvoid@silica@silicon (CVSS) nanospheres and cross-linked carboxymethyl cellulose and citric acid polymer binder (c-CMC-CA). Due to the additional protection from the silica layer, CVSS is superior to the carbon@void@silicon (CVS) electrode in terms of long-term cyclability. The as-prepared all-integrated CVSS electrode exhibits high mechanical strength, which can be ascribed to the high adhesivity and ductility of c-CMC-CA binder and the strong binding energy between CVSS and c-CMC-CA, as calculated based on density functional theory (DFT). This electrode exhibits a high reversible capacity of 1640 mA h g-1 after 100 cycles at a current density of 1 A g-1 , high rate performance, and long-term cycling stability with 84.6% capacity retention after 1000 cycles at 5 A g-1
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|a Journal Article
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|a all-integrated electrodes
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|a binding energy
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|a double-shelled-yolk-structured
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|a lithium-ion batteries
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|a multicomponent interlinking
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|a Tai, Zhixin
|e verfasserin
|4 aut
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|a Zhou, Tengfei
|e verfasserin
|4 aut
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|a Sencadas, Vitor
|e verfasserin
|4 aut
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|a Zhang, Jian
|e verfasserin
|4 aut
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|a Zhang, Lei
|e verfasserin
|4 aut
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1 |
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|a Konstantinov, Konstantin
|e verfasserin
|4 aut
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1 |
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|a Guo, Zaiping
|e verfasserin
|4 aut
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| 700 |
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|a Liu, Hua Kun
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 29(2017), 44 vom: 21. Nov.
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:29
|g year:2017
|g number:44
|g day:21
|g month:11
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|u http://dx.doi.org/10.1002/adma.201703028
|3 Volltext
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