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231225s2017 xx |||||o 00| ||eng c |
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|a 10.1002/adma.201606796
|2 doi
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|a pubmed24n0913.xml
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|a (NLM)28714071
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|a DE-627
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|e rakwb
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|a eng
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|a Shen, Jianlei
|e verfasserin
|4 aut
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|a Humidity-Responsive Single-Nanoparticle-Layer Plasmonic Films
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|c 2017
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Completed 18.07.2018
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|a Date Revised 01.10.2020
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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|a 2D materials possess many interesting properties, and have shown great application potentials. In this work, the development of humidity-responsive, 2D plasmonic nanostructures with switchable chromogenic properties upon wetting-dewetting transitions is reported. By exploiting DNA hybridization-directed anchoring of gold nanoparticles (AuNPs) on substrates, a series of single-nanoparticle-layer (SNL) plasmonic films is fabricated. Due to the collective plasmonic responses in SNL, these ultrathin 2D films display rapid and reversible red-blue color change upon the wetting-dewetting transition, suggesting that hydration-induced microscopic plasmonic coupling between AuNPs is replicated in the macroscopic, centimeter-scale films. It is also found that hydration finely tunes the electric field distribution between AuNPs in the SNL film, based on which responsive surface-enhanced Raman scattering substrates with spatially homogeneous hot spots are developed. Thus it is expected that DNA-mediated 2D SNL structures open new avenues for designing miniaturized plasmonic nanodevices with various applications
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|a Journal Article
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|a DNA
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|a chromogenic films
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|a gold nanoparticles
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|a plasmon coupling
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|a single nanoparticle layers
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|a Luan, Binquan
|e verfasserin
|4 aut
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|a Pei, Hao
|e verfasserin
|4 aut
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|a Yang, Zaixing
|e verfasserin
|4 aut
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|a Zuo, Xiaolei
|e verfasserin
|4 aut
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|a Liu, Gang
|e verfasserin
|4 aut
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|a Shi, Jiye
|e verfasserin
|4 aut
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|a Wang, Lihua
|e verfasserin
|4 aut
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|a Zhou, Ruhong
|e verfasserin
|4 aut
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|a Cheng, Wenlong
|e verfasserin
|4 aut
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|a Fan, Chunhai
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 29(2017), 35 vom: 01. Sept.
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:29
|g year:2017
|g number:35
|g day:01
|g month:09
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|u http://dx.doi.org/10.1002/adma.201606796
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