Humidity-Responsive Single-Nanoparticle-Layer Plasmonic Films

© 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 29(2017), 35 vom: 01. Sept.
1. Verfasser: Shen, Jianlei (VerfasserIn)
Weitere Verfasser: Luan, Binquan, Pei, Hao, Yang, Zaixing, Zuo, Xiaolei, Liu, Gang, Shi, Jiye, Wang, Lihua, Zhou, Ruhong, Cheng, Wenlong, Fan, Chunhai
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2017
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article DNA chromogenic films gold nanoparticles plasmon coupling single nanoparticle layers
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520 |a 2D materials possess many interesting properties, and have shown great application potentials. In this work, the development of humidity-responsive, 2D plasmonic nanostructures with switchable chromogenic properties upon wetting-dewetting transitions is reported. By exploiting DNA hybridization-directed anchoring of gold nanoparticles (AuNPs) on substrates, a series of single-nanoparticle-layer (SNL) plasmonic films is fabricated. Due to the collective plasmonic responses in SNL, these ultrathin 2D films display rapid and reversible red-blue color change upon the wetting-dewetting transition, suggesting that hydration-induced microscopic plasmonic coupling between AuNPs is replicated in the macroscopic, centimeter-scale films. It is also found that hydration finely tunes the electric field distribution between AuNPs in the SNL film, based on which responsive surface-enhanced Raman scattering substrates with spatially homogeneous hot spots are developed. Thus it is expected that DNA-mediated 2D SNL structures open new avenues for designing miniaturized plasmonic nanodevices with various applications 
650 4 |a Journal Article 
650 4 |a DNA 
650 4 |a chromogenic films 
650 4 |a gold nanoparticles 
650 4 |a plasmon coupling 
650 4 |a single nanoparticle layers 
700 1 |a Luan, Binquan  |e verfasserin  |4 aut 
700 1 |a Pei, Hao  |e verfasserin  |4 aut 
700 1 |a Yang, Zaixing  |e verfasserin  |4 aut 
700 1 |a Zuo, Xiaolei  |e verfasserin  |4 aut 
700 1 |a Liu, Gang  |e verfasserin  |4 aut 
700 1 |a Shi, Jiye  |e verfasserin  |4 aut 
700 1 |a Wang, Lihua  |e verfasserin  |4 aut 
700 1 |a Zhou, Ruhong  |e verfasserin  |4 aut 
700 1 |a Cheng, Wenlong  |e verfasserin  |4 aut 
700 1 |a Fan, Chunhai  |e verfasserin  |4 aut 
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773 1 8 |g volume:29  |g year:2017  |g number:35  |g day:01  |g month:09 
856 4 0 |u http://dx.doi.org/10.1002/adma.201606796  |3 Volltext 
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