Ultrafast Formation of Amorphous Bimetallic Hydroxide Films on 3D Conductive Sulfide Nanoarrays for Large-Current-Density Oxygen Evolution Electrocatalysis

© 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 29(2017), 22 vom: 07. Juni
1. Verfasser: Zou, Xu (VerfasserIn)
Weitere Verfasser: Liu, Yipu, Li, Guo-Dong, Wu, Yuanyuan, Liu, Da-Peng, Li, Wang, Li, Hai-Wen, Wang, Dejun, Zhang, Yu, Zou, Xiaoxin
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2017
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article composite materials large current density oxygen evolution reaction, electrocatalysis
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500 |a Date Revised 30.09.2020 
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520 |a Developing nonprecious oxygen evolution electrocatalysts that can work well at large current densities is of primary importance in a viable water-splitting technology. Herein, a facile ultrafast (5 s) synthetic approach is reported that produces a novel, efficient, non-noble metal oxygen-evolution nano-electrocatalyst that is composed of amorphous Ni-Fe bimetallic hydroxide film-coated, nickel foam (NF)-supported, Ni3 S2 nanosheet arrays. The composite nanomaterial (denoted as Ni-Fe-OHNi3 S2 /NF) shows highly efficient electrocatalytic activity toward oxygen evolution reaction (OER) at large current densities, even in the order of 1000 mA cm-2 . Ni-Fe-OH@Ni3 S2 /NF also gives an excellent catalytic stability toward OER both in 1 m KOH solution and in 30 wt% KOH solution. Further experimental results indicate that the effective integration of high catalytic reactivity, high structural stability, and high electronic conductivity into a single material system makes Ni-Fe-OH@Ni3 S2 /NF a remarkable catalytic ability for OER at large current densities 
650 4 |a Journal Article 
650 4 |a composite materials 
650 4 |a large current density 
650 4 |a oxygen evolution reaction, electrocatalysis 
700 1 |a Liu, Yipu  |e verfasserin  |4 aut 
700 1 |a Li, Guo-Dong  |e verfasserin  |4 aut 
700 1 |a Wu, Yuanyuan  |e verfasserin  |4 aut 
700 1 |a Liu, Da-Peng  |e verfasserin  |4 aut 
700 1 |a Li, Wang  |e verfasserin  |4 aut 
700 1 |a Li, Hai-Wen  |e verfasserin  |4 aut 
700 1 |a Wang, Dejun  |e verfasserin  |4 aut 
700 1 |a Zhang, Yu  |e verfasserin  |4 aut 
700 1 |a Zou, Xiaoxin  |e verfasserin  |4 aut 
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773 1 8 |g volume:29  |g year:2017  |g number:22  |g day:07  |g month:06 
856 4 0 |u http://dx.doi.org/10.1002/adma.201700404  |3 Volltext 
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