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250920s2025 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202504932
|2 doi
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|a pubmed25n1574.xml
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|a (NLM)40589174
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|a eng
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|a Bae, Juna
|e verfasserin
|4 aut
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|a Zeolite Structure Direction
|b Metals with a Dual Role as Amine Coordinators and Siloxy Connectors
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|c 2025
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Revised 19.09.2025
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2025 Wiley‐VCH GmbH.
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|a Innovation in the synthesis of new zeolites is achieved primarily through the use of costly novel organic compounds as structure-directing agents (SDAs). Here, a novel type of structure-direction based on a metal-amine coordination polymer leading to a 3-dimensional silicate-based hybrid material, LEU-1, is presented. The Zn-amine polymer not only serves as an SDA, but also plays a practical role in extending the inorganic connectivity in the form of Zn-O-Si bonds. This dual-role mechanism leads to unique hybrids with huge potential for creating zeolite-like materials. It is demonstrated that by using the silicate layer in LEU-1 as a platform, two novel pure-silica zeolites can be generated. This synthesis strategy, rooted in the coordination diversity of metal-amines, opens the door to more novel zeolite structures
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|a Journal Article
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|a dual‐role of metal ions
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4 |
|a organic‐inorganic hybrid materials
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| 650 |
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4 |
|a structure‐directing agents
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| 650 |
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4 |
|a syntheses
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| 650 |
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4 |
|a zeolites
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| 700 |
1 |
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|a Plessers, Dieter
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Ivanushkin, Gleb
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Bugaev, Aram
|e verfasserin
|4 aut
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| 700 |
1 |
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|a McCusker, Lynne B
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Dusselier, Michiel
|e verfasserin
|4 aut
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| 773 |
0 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 37(2025), 37 vom: 27. Sept., Seite e2504932
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnas
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| 773 |
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|g volume:37
|g year:2025
|g number:37
|g day:27
|g month:09
|g pages:e2504932
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|u http://dx.doi.org/10.1002/adma.202504932
|3 Volltext
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