General Prelithiation Approaches and the Corresponding Full Cell Design

© 2025 Wiley‐VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - (2025) vom: 06. Aug., Seite e08874
1. Verfasser: Song, Changsheng (VerfasserIn)
Weitere Verfasser: Zhang, Ce, Yuan, Qunyao, Gu, Yuanfan, Hou, Junyu, Zhao, Jie
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2025
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article Review initial Coulombic efficiency liquid and solid‐state lithium‐ion batteries prelithiation technology
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520 |a Prelithiation technology is widely regarded as an effective strategy to enhance the energy density and extend the cycle life of lithium-ion batteries (LIBs). The principle of prelithiation is to introduce additional active Li+, thereby compensating for Li losses during initial charging and long-term cycling. However, the current summaries of various prelithiation approaches are predominantly focused on liquid LIBs, with limited reviews available on solid-state LIBs. Compared to liquid LIBs, solid-state LIBs not only face uniformity issues caused by the uneven mixing of active materials and Li sources during prelithiation, but also encounter severe kinetic challenges arising from rigid solid-solid interface contact. Here, various prelithiation techniques are first integrated and the dynamic correlation between the prelithiation of each component in a full cell and its electrochemical performance is systematically introduced. Furthermore, the challenges of prelithiation techniques in solid-state LIBs in terms of solid-solid interface and Li+ transport are discussed. Finally, these prelithiation technologies are expected to be extended to the design of other premetallation agents, which guide the development of high-energy and high-safety energy storage systems 
650 4 |a Journal Article 
650 4 |a Review 
650 4 |a initial Coulombic efficiency 
650 4 |a liquid and solid‐state lithium‐ion batteries 
650 4 |a prelithiation technology 
700 1 |a Zhang, Ce  |e verfasserin  |4 aut 
700 1 |a Yuan, Qunyao  |e verfasserin  |4 aut 
700 1 |a Gu, Yuanfan  |e verfasserin  |4 aut 
700 1 |a Hou, Junyu  |e verfasserin  |4 aut 
700 1 |a Zhao, Jie  |e verfasserin  |4 aut 
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