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|a 10.1002/adma.202412432
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|a eng
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|a Zhu, Xin
|e verfasserin
|4 aut
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|a Large-Area Metal-Organic Framework Glasses for Efficient X-Ray Detection
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|c 2024
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Revised 19.12.2024
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2024 Wiley‐VCH GmbH.
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|a Cutting-edge techniques utilizing continuous films made from pure, novel semiconductive materials offer promising pathways to achieve high performance and cost-effectiveness for X-ray detection. Semiconductive metal-organic framework (MOF) glass films are known for their remarkably smooth surface morphology, straightforward synthesis, and capability for large-area fabrication, presenting a new direction for high-performance X-ray detectors. Here, a novel material centered on MOF glasses for highly uniform glass film fabrication customized for X-ray detection is introduced. MOF glasses, composed of zinc and imidazole derivatives, enable the transition from solid to liquid at low temperatures, facilitating the straightforward preparation of large-area and continuous MOF films with high mobility for X-ray device fabrication. Remarkably, MOF glass detectors demonstrate an exceptional sensitivity of 112.8 µC Gyair -1 cm-2 and a detection limit of 0.41 µGyair s-1, making them one of the most sensitive and with the best detection limits reported to date for MOF X-ray detectors. Clear X-ray images are successfully conducted using these developed MOF glass detectors for the first time. This breakthrough in X-ray sensitivity, and detection limit along with the spatial imaging resolution establishes a new standard for developing large-area and efficient MOF-based X-ray detectors with practical applications in medical and security screening
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|a Journal Article
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|a X‐ray detection
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|a large‐area film
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|a metal–organic framework glasses
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|a semiconductor MOF
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1 |
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|a He, Tengjiao
|e verfasserin
|4 aut
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1 |
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|a Song, Xin
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Shekhah, Osama
|e verfasserin
|4 aut
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|a Thomas, Simil
|e verfasserin
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|a Jiang, Hao
|e verfasserin
|4 aut
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|a Wu, Wentao
|e verfasserin
|4 aut
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| 700 |
1 |
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|a He, Tengyue
|e verfasserin
|4 aut
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|a Guillerm, Vincent
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Shkurenko, Aleksander
|e verfasserin
|4 aut
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|a Wang, Jian-Xin
|e verfasserin
|4 aut
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1 |
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|a Alshareef, Husam N
|e verfasserin
|4 aut
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1 |
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|a Bakr, Osman M
|e verfasserin
|4 aut
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|a Eddaoudi, Mohamed
|e verfasserin
|4 aut
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|a Mohammed, Omar F
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 51 vom: 17. Dez., Seite e2412432
|w (DE-627)NLM098206397
|x 1521-4095
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|g volume:36
|g year:2024
|g number:51
|g day:17
|g month:12
|g pages:e2412432
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|u http://dx.doi.org/10.1002/adma.202412432
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