Enabling 2D Electron Gas with High Room-Temperature Electron Mobility Exceeding 100 cm2 Vs-1 at a Perovskite Oxide Interface

© 2024 The Author(s). Advanced Materials published by Wiley‐VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 36(2024), 50 vom: 02. Dez., Seite e2409076
1. Verfasser: Hoffmann, Georg (VerfasserIn)
Weitere Verfasser: Zupancic, Martina, Riaz, Aysha A, Kalha, Curran, Schlueter, Christoph, Gloskovskii, Andrei, Regoutz, Anna, Albrecht, Martin, Nordlander, Johanna, Bierwagen, Oliver
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2024
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article 2D electron gas BaSnO3 LaInO3 high mobility molecular beam epitaxy perovskite oxides
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520 |a In perovskite oxide heterostructures, bulk functional properties coexist with emergent physical phenomena at epitaxial interfaces. Notably, charge transfer at the interface between two insulating oxide layers can lead to the formation of a 2D electron gas (2DEG) with possible applications in, e.g., high-electron-mobility transistors and ferroelectric field-effect transistors. So far, the realization of oxide 2DEGs is, however, largely limited to the interface between the single-crystal substrate and epitaxial film, preventing their deliberate placement inside a larger device architecture. Additionally, the substrate-limited quality of perovskite oxide interfaces hampers room-temperature (RT) 2DEG performance due to notoriously low electron mobility. In this work, the controlled creation of an interfacial 2DEG at the epitaxial interface between perovskite oxides BaSnO3 and LaInO3 is demonstrated with enhanced RT electron mobility values up to 119 cm2 Vs-1-the highest RT value reported so far for a perovskite oxide 2DEG. Using a combination of state-of-the-art deposition modes during oxide molecular beam epitaxy, this approach opens up another degree of freedom in optimization and in situ control of the interface between two epitaxial oxide layers away from the substrate interface. Thus this approach is expected to apply to the general class of perovskite oxide 2DEG systems and to enable their improved compatibility with novel device concepts and integration across materials platforms 
650 4 |a Journal Article 
650 4 |a 2D electron gas 
650 4 |a BaSnO3 
650 4 |a LaInO3 
650 4 |a high mobility 
650 4 |a molecular beam epitaxy 
650 4 |a perovskite oxides 
700 1 |a Zupancic, Martina  |e verfasserin  |4 aut 
700 1 |a Riaz, Aysha A  |e verfasserin  |4 aut 
700 1 |a Kalha, Curran  |e verfasserin  |4 aut 
700 1 |a Schlueter, Christoph  |e verfasserin  |4 aut 
700 1 |a Gloskovskii, Andrei  |e verfasserin  |4 aut 
700 1 |a Regoutz, Anna  |e verfasserin  |4 aut 
700 1 |a Albrecht, Martin  |e verfasserin  |4 aut 
700 1 |a Nordlander, Johanna  |e verfasserin  |4 aut 
700 1 |a Bierwagen, Oliver  |e verfasserin  |4 aut 
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773 1 8 |g volume:36  |g year:2024  |g number:50  |g day:02  |g month:12  |g pages:e2409076 
856 4 0 |u http://dx.doi.org/10.1002/adma.202409076  |3 Volltext 
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