Bifunctional system constructed by NiCu-F/DSA electrode self-coupling for efficient removal of ammonia nitrogen from landfill leachate

Landfill leachates containing high concentrations of ammonia nitrogen, due to its strong toxicity, large discharge and great environmental hazard, is in urgent need of efficient cleaning treatment. In this work, Ni1Cu0.25-F/DSA catalytic electrode was prepared via electrodeposition by means of fluor...

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Veröffentlicht in:Environmental technology. - 1993. - (2024) vom: 16. Okt., Seite 1-15
1. Verfasser: Li, Bing (VerfasserIn)
Weitere Verfasser: Tong, Xing, Wang, Hailong, Zhou, Luanqi, Li, Qiming, Yao, Na, Zhang, Meng, Zhang, Huimin
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2024
Zugriff auf das übergeordnete Werk:Environmental technology
Schlagworte:Journal Article Electrochemical oxidation ammonia oxidation reaction bifunctional system denitrification landfill leachate
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520 |a Landfill leachates containing high concentrations of ammonia nitrogen, due to its strong toxicity, large discharge and great environmental hazard, is in urgent need of efficient cleaning treatment. In this work, Ni1Cu0.25-F/DSA catalytic electrode was prepared via electrodeposition by means of fluorination-induced surface reconstruction. The surface of electrode was determined to be a porous sponge-like structure by physical characterizations. The electrode exhibited a superior ammonia oxidation reaction (AOR) activity and stability by a series of electrochemical tests. On this basis, a Ni1Cu0.25-F/DSA || Ni1Cu0.25-F/DSA bifunctional system was developed for efficient removal of ammonia nitrogen in landfill leachate. The results of denitrification experiment indicated that the removal efficiency of NH4+-N and TN were 99.89% and 68.9%, respectively, when the electrolytic cell potential was 1.7 V, pH was 13 and the initial ammonia concentration was 600 mg L-1. The NH4+-N removal efficiency remained above 95% after the cyclic denitrification experiment lasting for 6 days, which validates the robust stability of the electrode 
650 4 |a Journal Article 
650 4 |a Electrochemical oxidation 
650 4 |a ammonia oxidation reaction 
650 4 |a bifunctional system 
650 4 |a denitrification 
650 4 |a landfill leachate 
700 1 |a Tong, Xing  |e verfasserin  |4 aut 
700 1 |a Wang, Hailong  |e verfasserin  |4 aut 
700 1 |a Zhou, Luanqi  |e verfasserin  |4 aut 
700 1 |a Li, Qiming  |e verfasserin  |4 aut 
700 1 |a Yao, Na  |e verfasserin  |4 aut 
700 1 |a Zhang, Meng  |e verfasserin  |4 aut 
700 1 |a Zhang, Huimin  |e verfasserin  |4 aut 
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773 1 8 |g year:2024  |g day:16  |g month:10  |g pages:1-15 
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