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|a 10.1021/acs.chemmater.4c01535
|2 doi
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|a DE-627
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|e rakwb
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|a eng
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|a Frandsen, Benjamin A
|e verfasserin
|4 aut
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|a A New Spin on Material Properties
|b Local Magnetic Structure in Functional and Quantum Materials
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|c 2024
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Revised 15.10.2024
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|a published: Electronic-eCollection
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|a Citation Status PubMed-not-MEDLINE
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|a © 2024 The Authors. Published by American Chemical Society.
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|a The past few decades have made clear that the properties and performances of emerging functional and quantum materials can depend strongly on their local atomic and/or magnetic structure, particularly when details of the local structure deviate from the long-range structure averaged over space and time. Traditional methods of structural refinement (e.g., Rietveld) are typically sensitive only to the average structure, creating a need for more advanced structural probes suitable for extracting information about structural correlations on short length- and time-scales. In this Perspective, we describe the importance of local magnetic structure in several classes of emerging materials and present the magnetic pair distribution function (mPDF) technique as a powerful tool for studying short-range magnetism from neutron total-scattering data. We then provide a selection of examples of mPDF analysis applied to magnetic materials of recent technological and fundamental interest, including the antiferromagnetic semiconductor MnTe, geometrically frustrated magnets, and iron-oxide magnetic nanoparticles. The rapid development of mPDF analysis since its formalization a decade ago puts this technique in a strong position for making continued impact in the study of local magnetism in emerging materials
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|a Journal Article
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|a Review
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|a Fischer, Henry E
|e verfasserin
|4 aut
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|i Enthalten in
|t Chemistry of materials : a publication of the American Chemical Society
|d 1998
|g 36(2024), 19 vom: 08. Okt., Seite 9089-9106
|w (DE-627)NLM098194763
|x 0897-4756
|7 nnns
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|g volume:36
|g year:2024
|g number:19
|g day:08
|g month:10
|g pages:9089-9106
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|u http://dx.doi.org/10.1021/acs.chemmater.4c01535
|3 Volltext
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|d 36
|j 2024
|e 19
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