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240926s2024 xx |||||o 00| ||eng c |
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|a 10.1021/acs.langmuir.4c02635
|2 doi
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|a eng
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|a Wang, Jiajia
|e verfasserin
|4 aut
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|a Enhanced Photocatalytic Hydrogen Production Activity Driven by TiO2/(MoP/CdS)
|b Insights from Powder Particles to Thin Films
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|c 2024
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|a Text
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|a ƒaComputermedien
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|a Date Revised 08.10.2024
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a Transitioning from powder photocatalysts to thin film photocatalysts is one of the necessary steps toward industrializing photocatalytic hydrogen production. Herein, we reported the integration of non-noble metal cocatalyst MoP decorated with TiO2 and CdS, forming TiO2/(MoP/CdS) for ultraviolet-visible light utilization. The designed powder TiO2/(MoP/CdS) composites achieved a superior hydrogen production rate of 42.2 mmol g-1 h-1, which is 30.1 times that of TiO2/CdS, performing the highest activity among the TiO2-CdS-based composite photocatalysts. Moreover, we fabricated a thin film from TiO2/(MoP/CdS) powder, which exhibited comparable photocatalytic activity for hydrogen production, achieving 35.5 mmol g-1 h-1 and maintaining long-term stability for 150 h. The outstanding performance was attributed to the ability of the TiO2/(MoP/CdS) composite photocatalysts to absorb both visible and ultraviolet light. Additionally, the heterojunction formed between TiO2 and CdS also played a significant role in the overall photocatalyst activity. This cost-effective catalyst holds promise for future large-scale industrial applications
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|a Journal Article
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1 |
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|a Tian, Jinfeng
|e verfasserin
|4 aut
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|a Han, Peng
|e verfasserin
|4 aut
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| 700 |
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|a Song, Lingxiao
|e verfasserin
|4 aut
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|a Wang, Wei
|e verfasserin
|4 aut
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| 700 |
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|a Lin, Keying
|e verfasserin
|4 aut
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|a Feng, Dong
|e verfasserin
|4 aut
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| 700 |
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|a Ma, Baojun
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Langmuir : the ACS journal of surfaces and colloids
|d 1999
|g 40(2024), 40 vom: 08. Okt., Seite 21161-21170
|w (DE-627)NLM098181009
|x 1520-5827
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|g volume:40
|g year:2024
|g number:40
|g day:08
|g month:10
|g pages:21161-21170
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|u http://dx.doi.org/10.1021/acs.langmuir.4c02635
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