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240923s2024 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202412007
|2 doi
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|a pubmed24n1546.xml
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|a (DE-627)NLM377951579
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|a (NLM)39308205
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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|a Liu, Yuanfeng
|e verfasserin
|4 aut
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|a Broadband Spin and Orbital Momentum Modulator Using Self-Assembled Nanostructures
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|c 2024
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Revised 23.09.2024
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|a published: Print-Electronic
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|a Citation Status Publisher
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|a © 2024 Wiley‐VCH GmbH.
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|a The structural symmetry of solids plays an important role in defining their linear and nonlinear optical properties. The quest for versatile, cost-effective, large-scale, and defect-free approaches and materials platforms for tailoring structural and optical properties on demand is underway since decades. A self-assembled spherulite material comprised of synthesized molecules with large dipole moments aligned azimuthally, forming a vortex polarity with spontaneously broken symmetry, is experimentally demonstrated. This unique self-assembled structure enables new linear and nonlinear light-matter interactions, including generating optical vortex beams with complex spin states and on-demand topological charges at the fundamental, doubled, and tripled frequencies. This work will likely enable numerous applications in areas such as high-dimensional quantum information processing with large capacity and high security, spatiotemporal optical vortices, and a novel optical manipulation and trapping platform
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|a Journal Article
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|a optical vortex
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|a orbital angular momentum
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|a spherulite
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|a vortex polarity
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|a Zhou, Le
|e verfasserin
|4 aut
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|a Guo, Mengfan
|e verfasserin
|4 aut
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|a Xu, Zongqi
|e verfasserin
|4 aut
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|a Ma, Jing
|e verfasserin
|4 aut
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|a Wen, Yongzheng
|e verfasserin
|4 aut
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|a Litchinitser, Natalia M
|e verfasserin
|4 aut
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|a Shen, Yang
|e verfasserin
|4 aut
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|a Sun, Jingbo
|e verfasserin
|4 aut
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|a Zhou, Ji
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g (2024) vom: 23. Sept., Seite e2412007
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g year:2024
|g day:23
|g month:09
|g pages:e2412007
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|u http://dx.doi.org/10.1002/adma.202412007
|3 Volltext
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