Broadband Spin and Orbital Momentum Modulator Using Self-Assembled Nanostructures

© 2024 Wiley‐VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - (2024) vom: 23. Sept., Seite e2412007
1. Verfasser: Liu, Yuanfeng (VerfasserIn)
Weitere Verfasser: Zhou, Le, Guo, Mengfan, Xu, Zongqi, Ma, Jing, Wen, Yongzheng, Litchinitser, Natalia M, Shen, Yang, Sun, Jingbo, Zhou, Ji
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2024
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article optical vortex orbital angular momentum spherulite vortex polarity
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520 |a The structural symmetry of solids plays an important role in defining their linear and nonlinear optical properties. The quest for versatile, cost-effective, large-scale, and defect-free approaches and materials platforms for tailoring structural and optical properties on demand is underway since decades. A self-assembled spherulite material comprised of synthesized molecules with large dipole moments aligned azimuthally, forming a vortex polarity with spontaneously broken symmetry, is experimentally demonstrated. This unique self-assembled structure enables new linear and nonlinear light-matter interactions, including generating optical vortex beams with complex spin states and on-demand topological charges at the fundamental, doubled, and tripled frequencies. This work will likely enable numerous applications in areas such as high-dimensional quantum information processing with large capacity and high security, spatiotemporal optical vortices, and a novel optical manipulation and trapping platform 
650 4 |a Journal Article 
650 4 |a optical vortex 
650 4 |a orbital angular momentum 
650 4 |a spherulite 
650 4 |a vortex polarity 
700 1 |a Zhou, Le  |e verfasserin  |4 aut 
700 1 |a Guo, Mengfan  |e verfasserin  |4 aut 
700 1 |a Xu, Zongqi  |e verfasserin  |4 aut 
700 1 |a Ma, Jing  |e verfasserin  |4 aut 
700 1 |a Wen, Yongzheng  |e verfasserin  |4 aut 
700 1 |a Litchinitser, Natalia M  |e verfasserin  |4 aut 
700 1 |a Shen, Yang  |e verfasserin  |4 aut 
700 1 |a Sun, Jingbo  |e verfasserin  |4 aut 
700 1 |a Zhou, Ji  |e verfasserin  |4 aut 
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