N/O Co-doped Porous Carbon with Controllable Porosity Synthesized via an All-in-One Step Method for a High-Rate-Performance Supercapacitor

A green and economical methodology to fabricate carbon-based materials with suitable pore size distributions is needed to achieve rapid electrolyte diffusion and improve the performance of supercapacitors. Here, a method combining in situ templates with self-activation and self-doping is proposed. B...

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Veröffentlicht in:Langmuir : the ACS journal of surfaces and colloids. - 1992. - 40(2024), 37 vom: 17. Sept., Seite 19665-19674
1. Verfasser: He, Chenweijia (VerfasserIn)
Weitere Verfasser: Yang, Guangjie, Ni, Liye, Yang, Haoqi, Peng, Yongshuo, Liu, Xiangdong, Li, Ping, Song, Cheng, He, Shuijian, Zhang, Qian
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2024
Zugriff auf das übergeordnete Werk:Langmuir : the ACS journal of surfaces and colloids
Schlagworte:Journal Article
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520 |a A green and economical methodology to fabricate carbon-based materials with suitable pore size distributions is needed to achieve rapid electrolyte diffusion and improve the performance of supercapacitors. Here, a method combining in situ templates with self-activation and self-doping is proposed. By variation of the molar ratio of magnesium folate and potassium folate, the pore size distribution was effectively adjusted. The optimal carbon materials (Kx) have a high specific surface area (1021-1676 m2 g-1) and hierarchical pore structure, which significantly promotes its excellent capacitive properties. Notably, K2 shows an excellent mass specific capacitance of 233 F g-1 at 0.1 A g-1. It still retained 113 F g-1 at 55 A g-1. The assembled symmetric supercapacitor exhibited an outstanding cyclic stability. It maintains 100% capacitance after 100 000 cycles at 10 A g-1. The symmetric supercapacitor demonstrated a maximum power density of 99.8 kW kg-1. This study focuses on the preparation of layered pore structures to provide insights into the sustainable design of carbon materials 
650 4 |a Journal Article 
700 1 |a Yang, Guangjie  |e verfasserin  |4 aut 
700 1 |a Ni, Liye  |e verfasserin  |4 aut 
700 1 |a Yang, Haoqi  |e verfasserin  |4 aut 
700 1 |a Peng, Yongshuo  |e verfasserin  |4 aut 
700 1 |a Liu, Xiangdong  |e verfasserin  |4 aut 
700 1 |a Li, Ping  |e verfasserin  |4 aut 
700 1 |a Song, Cheng  |e verfasserin  |4 aut 
700 1 |a He, Shuijian  |e verfasserin  |4 aut 
700 1 |a Zhang, Qian  |e verfasserin  |4 aut 
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