|
|
|
|
| LEADER |
01000caa a22002652 4500 |
| 001 |
NLM373693443 |
| 003 |
DE-627 |
| 005 |
20240808233224.0 |
| 007 |
cr uuu---uuuuu |
| 008 |
240617s2024 xx |||||o 00| ||eng c |
| 024 |
7 |
|
|a 10.1002/adma.202403873
|2 doi
|
| 028 |
5 |
2 |
|a pubmed24n1495.xml
|
| 035 |
|
|
|a (DE-627)NLM373693443
|
| 035 |
|
|
|a (NLM)38881289
|
| 040 |
|
|
|a DE-627
|b ger
|c DE-627
|e rakwb
|
| 041 |
|
|
|a eng
|
| 100 |
1 |
|
|a Gorobtsov, Oleg Yu
|e verfasserin
|4 aut
|
| 245 |
1 |
0 |
|a Spontaneous Supercrystal Formation During a Strain-Engineered Metal-Insulator Transition
|
| 264 |
|
1 |
|c 2024
|
| 336 |
|
|
|a Text
|b txt
|2 rdacontent
|
| 337 |
|
|
|a ƒaComputermedien
|b c
|2 rdamedia
|
| 338 |
|
|
|a ƒa Online-Ressource
|b cr
|2 rdacarrier
|
| 500 |
|
|
|a Date Revised 08.08.2024
|
| 500 |
|
|
|a published: Print-Electronic
|
| 500 |
|
|
|a Citation Status PubMed-not-MEDLINE
|
| 520 |
|
|
|a © 2024 Wiley‐VCH GmbH.
|
| 520 |
|
|
|a Mott metal-insulator transitions possess electronic, magnetic, and structural degrees of freedom promising next-generation energy-efficient electronics. A previously unknown, hierarchically ordered, and anisotropic supercrystal state is reported and its intrinsic formation characterized in-situ during a Mott transition in a Ca2RuO4 thin film. Machine learning-assisted X-ray nanodiffraction together with cryogenic electron microscopy reveal multi-scale periodic domain formation at and below the film transition temperature (TFilm ≈ 200-250 K) and a separate anisotropic spatial structure at and above TFilm. Local resistivity measurements imply an intrinsic coupling of the supercrystal orientation to the material's anisotropic conductivity. These findings add a new degree of complexity to the physical understanding of Mott transitions, opening opportunities for designing materials with tunable electronic properties
|
| 650 |
|
4 |
|a Journal Article
|
| 650 |
|
4 |
|a coherent X‐ray diffraction
|
| 650 |
|
4 |
|a nanomaterials
|
| 650 |
|
4 |
|a quantum materials
|
| 650 |
|
4 |
|a supercrystals
|
| 650 |
|
4 |
|a thin films
|
| 700 |
1 |
|
|a Miao, Ludi
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Shao, Ziming
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Tan, Yueze
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Schnitzer, Noah
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Goodge, Berit Hansen
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Ruf, Jacob
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Weinstock, Daniel
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Cherukara, Mathew
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Holt, Martin Victor
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Nair, Hari
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Chen, Long-Qing
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Kourkoutis, Lena Fitting
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Schlom, Darrell G
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Shen, Kyle M
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Singer, Andrej
|e verfasserin
|4 aut
|
| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 32 vom: 02. Aug., Seite e2403873
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
|
| 773 |
1 |
8 |
|g volume:36
|g year:2024
|g number:32
|g day:02
|g month:08
|g pages:e2403873
|
| 856 |
4 |
0 |
|u http://dx.doi.org/10.1002/adma.202403873
|3 Volltext
|
| 912 |
|
|
|a GBV_USEFLAG_A
|
| 912 |
|
|
|a SYSFLAG_A
|
| 912 |
|
|
|a GBV_NLM
|
| 912 |
|
|
|a GBV_ILN_350
|
| 951 |
|
|
|a AR
|
| 952 |
|
|
|d 36
|j 2024
|e 32
|b 02
|c 08
|h e2403873
|