Extreme Fast Charging of Lithium Metal Batteries Enabled by a Molten-Salt-Derived Nanocrystal Interphase

© 2024 Wiley‐VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 36(2024), 32 vom: 05. Aug., Seite e2404630
1. Verfasser: Wu, Wei (VerfasserIn)
Weitere Verfasser: Niu, Fang, Sun, Chuankui, Wang, Qingrong, Wang, Man, Wang, Jun, Deng, Yonghong, Ning, De, Li, Wenjie, Zhang, Jie, Chen, Ming, Cheng, Hui-Ming, Yang, Chunlei
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2024
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article anode dendrite extreme fast charging lithium metal battery roll‐to‐roll solid electrolyte interphase
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520 |a The extreme fast charging performance of lithium metal batteries (LMBs) with a long life is an important focus in the development of next-generation battery technologies. The friable solid electrolyte interphase and dendritic lithium growth are major problems. The formation of an inorganic nanocrystal-dominant interphase produced by preimmersing the Li in molten lithium bis(fluorosulfonyl)imide that suppresses the overgrowth of the usual interphase is reported. Its high surface modulus combined with fast Li+ diffusivity enables a reversible dendrite-proof deposition under ultrahigh-rate conditions. It gives a record-breaking cumulative plating/stripping capacity of >240 000 mAh cm-2 at 30 mA cm-230 mAh cm-2 for a symmetric cell and an extreme fast charging performance at 6 C for 500 cycles for a Li||LiCoO2 full cell with a high-areal-capacity, thus expanding the use of LMBs to high-loading and power-intensive scenarios. Its usability both in roll-to-roll production and in different electrolytes indicating the scalable and industrial potential of this process for high-performance LMBs 
650 4 |a Journal Article 
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650 4 |a dendrite 
650 4 |a extreme fast charging 
650 4 |a lithium metal battery 
650 4 |a roll‐to‐roll 
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700 1 |a Niu, Fang  |e verfasserin  |4 aut 
700 1 |a Sun, Chuankui  |e verfasserin  |4 aut 
700 1 |a Wang, Qingrong  |e verfasserin  |4 aut 
700 1 |a Wang, Man  |e verfasserin  |4 aut 
700 1 |a Wang, Jun  |e verfasserin  |4 aut 
700 1 |a Deng, Yonghong  |e verfasserin  |4 aut 
700 1 |a Ning, De  |e verfasserin  |4 aut 
700 1 |a Li, Wenjie  |e verfasserin  |4 aut 
700 1 |a Zhang, Jie  |e verfasserin  |4 aut 
700 1 |a Chen, Ming  |e verfasserin  |4 aut 
700 1 |a Cheng, Hui-Ming  |e verfasserin  |4 aut 
700 1 |a Yang, Chunlei  |e verfasserin  |4 aut 
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773 1 8 |g volume:36  |g year:2024  |g number:32  |g day:05  |g month:08  |g pages:e2404630 
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