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240416s2024 xx |||||o 00| ||eng c |
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|a 10.2166/wst.2024.098
|2 doi
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|a pubmed24n1378.xml
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|a (DE-627)NLM371092272
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|a (NLM)38619897
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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|a Zhang, Longbin
|e verfasserin
|4 aut
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|a Ascorbic acid enhanced the circulation between Fe(II) and Fe(III) in peroxymonosulfate system for fluoranthene degradation
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|c 2024
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Completed 17.04.2024
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|a Date Revised 17.04.2024
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|a published: Print-Electronic
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|a Citation Status MEDLINE
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|a © 2024 The Authors This is an Open Access article distributed under the terms of the Creative Commons Attribution Licence (CC BY 4.0), which permits copying, adaptation and redistribution, provided the original work is properly cited (http://creativecommons.org/licenses/by/4.0/).
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|a In this research, ascorbic acid (AA) was used to enhance Fe(II)/Fe(III)-activated permonosulfate (PMS) systems for the degradation of fluoranthene (FLT). AA enhanced the production of ROS in both PMS/Fe(II) and PMS/Fe(III) systems through chelation and reduction and thus improved the degradation performance of FLT. The optimal molar ratio in PMS/Fe(II)/AA/FLT and PMS/Fe(III)/AA/FLT processes were 2/2/4/1 and 5/10/5/1, respectively. In addition, the experimental results on the effect of FLT degradation under different groundwater matrixes indicated that PMS/Fe(III)/AA system was more adaptable to different water quality conditions than the PMS/Fe(II)/AA system. SO4·- was the major reactive oxygen species (ROS) responsible for FLT removal through the probe and scavenging tests in both systems. Furthermore, the degradation intermediates of FLT were analyzed using gas chromatograph-mass spectrometry (GC-MS), and the probable degradation pathways of FLT degradation were proposed. In addition, the removal of FLT was also tested in actual groundwater and the results showed that by increasing the dose and pre-adjusting the solution pH, 88.8 and 100% of the FLT was removed for PMS/Fe(II)/AA and PMS/Fe(III)/AA systems. The above experimental results demonstrated that PMS/Fe(II)/AA and PMS/Fe(III)/AA processes have a great perspective in practice for the rehabilitation of FLT-polluted groundwater
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|a Journal Article
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|a Fe(II)
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|a Fe(III)
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|a ascorbic acid
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|a peroxymonosulfate
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|a remediation
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|a peroxymonosulfate
|2 NLM
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|a 22047-43-4
|2 NLM
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|a Ferric Compounds
|2 NLM
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|a fluoranthene
|2 NLM
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|a 360UOL779Z
|2 NLM
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|a Reactive Oxygen Species
|2 NLM
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|a Water Pollutants, Chemical
|2 NLM
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|a Peroxides
|2 NLM
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|a Ferrous Compounds
|2 NLM
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|a Fluorenes
|2 NLM
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| 700 |
1 |
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|a Gao, Jianxiong
|e verfasserin
|4 aut
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1 |
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|a Liu, Yulong
|e verfasserin
|4 aut
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|a Zhou, Zhengyuan
|e verfasserin
|4 aut
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|a Sheng, Xianxian
|e verfasserin
|4 aut
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|a Li, Dexiao
|e verfasserin
|4 aut
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|a Chen, Yuantian
|e verfasserin
|4 aut
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|a Lyu, Shuguang
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Water science and technology : a journal of the International Association on Water Pollution Research
|d 1986
|g 89(2024), 7 vom: 14. Apr., Seite 1682-1700
|w (DE-627)NLM098149431
|x 0273-1223
|7 nnns
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| 773 |
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|g volume:89
|g year:2024
|g number:7
|g day:14
|g month:04
|g pages:1682-1700
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|u http://dx.doi.org/10.2166/wst.2024.098
|3 Volltext
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|d 89
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