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240415s2024 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202312685
|2 doi
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|a pubmed25n1236.xml
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|a eng
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|a Li, Huan
|e verfasserin
|4 aut
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|a Mn-Based Mullites for Environmental and Energy Applications
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|c 2024
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|a Text
|b txt
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Revised 24.05.2024
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2024 Wiley‐VCH GmbH.
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|a Mn-based mullite oxides AMn2O5 (A = lanthanide, Y, Bi) is a novel type of ternary catalyst in terms of their electronic and geometric structures. The coexistence of pyramid Mn3+-O and octahedral Mn4+-O makes the d-orbital selectively active toward various catalytic reactions. The alternative edge- and corner-sharing stacking configuration constructs the confined active sites and abundant active oxygen species. As a result, they tend to show superior catalytic behaviors and thus gain great attention in environmental treatment and energy conversion and storage. In environmental applications, Mn-based mullites have been demonstrated to be highly active toward low-temperature oxidization of CO, NO, volatile organic compounds (VOCs), etc. Recent research further shows that mullites decompose O3 and ozonize VOCs from -20 °C to room temperature. Moreover, mullites enhance oxygen reduction reactions (ORR) and sulfur reduction reactions (SRR), critical kinetic steps in air-battery and Li-S batteries, respectively. Their distinctive structures also facilitate applications in gas-sensitive sensing, ionic conduction, high mobility dielectrics, oxygen storage, piezoelectricity, dehydration, H2O2 decomposition, and beyond. A comprehensive review from basic physicochemical properties to application certainly not only gains a full picture of mullite oxides but also provides new insights into designing heterogeneous catalysts
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|a Journal Article
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|a Review
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|a Mn‐based mullites
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|a energy storage and conversion
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|a pollutant gaseous treatment
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|a room temperature catalysis
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|a sensor materials
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|a Wang, Wanying
|e verfasserin
|4 aut
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|a Xu, Jinchao
|e verfasserin
|4 aut
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| 700 |
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|a Wang, Ansheng
|e verfasserin
|4 aut
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|a Wan, Xiang
|e verfasserin
|4 aut
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| 700 |
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|a Yang, Liyuan
|e verfasserin
|4 aut
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| 700 |
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|a Zhao, Haojun
|e verfasserin
|4 aut
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| 700 |
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|a Shan, Qingyu
|e verfasserin
|4 aut
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| 700 |
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|a Zhao, Chunning
|e verfasserin
|4 aut
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| 700 |
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|a Sun, Shuhui
|e verfasserin
|4 aut
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| 700 |
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|a Wang, Weichao
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 21 vom: 15. Mai, Seite e2312685
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnas
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|g volume:36
|g year:2024
|g number:21
|g day:15
|g month:05
|g pages:e2312685
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|u http://dx.doi.org/10.1002/adma.202312685
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