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|a 10.1002/adma.202401550
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|a eng
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|a Zhang, Hanxue
|e verfasserin
|4 aut
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|a Stretchable Electrodes with Interfacial Percolation Network
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|c 2024
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|a Text
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|a ƒaComputermedien
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|a Date Revised 26.06.2024
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2024 Wiley‐VCH GmbH.
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|a Stretchable electrodes are an essential component that determines the functionality and reliability of stretchable electronics, but face the challenge of balancing conductivity and stretchability. This work proposes a new conducting concept called the interfacial percolation network (PN) that results in stretchable electrodes with high conductivity, large stretchability, and high stability. The interfacial PN is composed of a 2D silver nanowires (AgNWs) PN and a protruding 3D AgNWs PN embedded on the surface and in the near-surface region of an elastic polymer matrix, respectively. The protruded PN is obtained by changing the arrangements of AgNWs from horizontal to quasi-vertical through introducing foreign polymer domains in the near-surface region of the polymer matrix. The resulting electrode achieves a conductivity of 13 500 S cm-1 and a stretchability of 660%. Its resistance changes under stretched conditions are orders of magnitude lower than those of conventional 2D PN and 2D + 3D PN. An interfacial PN electrode made from liquid metal remained its conductivity at 46 750 S cm-1 after the electrode underwent multiple stretch-release cycles with a deformation of >600%. The concept of interfacial PN provides fruitful implications for the design of stretchable electronics
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|a Journal Article
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|a AgNWs
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|a interfacial percolation network
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|a liquid metal
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|a stretchable electrode
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|a Shao, Yan
|e verfasserin
|4 aut
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|a Xia, Rui
|e verfasserin
|4 aut
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|a Chen, Guoli
|e verfasserin
|4 aut
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|a Xiang, Xinyue
|e verfasserin
|4 aut
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|a Yu, Yanhao
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 26 vom: 27. Juni, Seite e2401550
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:36
|g year:2024
|g number:26
|g day:27
|g month:06
|g pages:e2401550
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|u http://dx.doi.org/10.1002/adma.202401550
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