A Solid-Liquid Bicontinuous Fiber with Strain-Insensitive Ionic Conduction

© 2024 Wiley‐VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 36(2024), 25 vom: 01. Juni, Seite e2402501
1. Verfasser: Ye, Huating (VerfasserIn)
Weitere Verfasser: Wu, Baohu, Sun, Shengtong, Wu, Peiyi
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2024
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article anti‐fatigue ionic conductors phase separation strain‐insensitive stretchable fibers
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520 |a Stretchable ionic conductors are crucial for enabling advanced iontronic devices to operate under diverse deformation conditions. However, when employed as interconnects, existing ionic conductors struggle to maintain stable ionic conduction under strain, hindering high-fidelity signal transmission. Here, it is shown that strain-insensitive ionic conduction can be achieved by creating a solid-liquid bicontinuous microstructure. A bicontinuous fiber from polymerization-induced phase separation, which contains a solid elastomer phase interpenetrated by a liquid ion-conducting phase, is fabricated. The spontaneous partitioning of dissolved salts leads to the formation of a robust self-wrinkled interface, fostering the development of highly tortuous ionic channels. Upon stretch, these meandering ionic channels are straightened, effectively enhancing ionic conductivity to counteract the strain effect. Remarkably, the fiber retains highly stable ionic conduction till fracture, with only 7% resistance increase at 200% strain. This approach presents a promising avenue for designing durable ionic cables capable of signal transmission with minimal strain-induced distortion 
650 4 |a Journal Article 
650 4 |a anti‐fatigue 
650 4 |a ionic conductors 
650 4 |a phase separation 
650 4 |a strain‐insensitive 
650 4 |a stretchable fibers 
700 1 |a Wu, Baohu  |e verfasserin  |4 aut 
700 1 |a Sun, Shengtong  |e verfasserin  |4 aut 
700 1 |a Wu, Peiyi  |e verfasserin  |4 aut 
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773 1 8 |g volume:36  |g year:2024  |g number:25  |g day:01  |g month:06  |g pages:e2402501 
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