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240328s2024 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202401659
|2 doi
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|a pubmed24n1476.xml
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|a (DE-627)NLM370234553
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|a (NLM)38533903
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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|a Wu, Baoyi
|e verfasserin
|4 aut
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|a Cephalopod-Inspired Chemical-Gated Hydrogel Actuation Systems for Information 3D-Encoding Display
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|c 2024
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Revised 20.07.2024
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2024 Wiley‐VCH GmbH.
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|a Cephalopods evolve the acetylcholine-gated actuation control function of their skin muscles, which enables their dynamic/static multimode display capacities for achieving perfectly spatial control over the colors/patterns on every inch of skin. Reproduction of artificial analogs that exhibit similar multimodal display is essential to reach advanced information three-dimensional (3D) encoding with higher security than the classic 2D-encoding strategy, but remains underdeveloped. The core difficulty is how to replicate such chemical-gated actuation control function into artificial soft actuating systems. Herein, this work proposes to develop azobenzene-functionalized poly(acrylamide) (PAAm) hydrogel systems, whose upper critical solution temperature (UCST) type actuation responsiveness can be intelligently programmed or even gated by the addition of hydrophilic α-cyclodextrin (α-CD) molecules for reversible association with pendant azobenzene moieties via supramolecular host-guest interactions. By employing such α-CD-gated hydrogel actuator as an analogue of cephalopods' skin muscle, biomimetic mechanically modulated multicolor fluorescent display systems are designed, which demonstrate a conceptually new α-CD-gated "thermal stimulation-hydrogel actuation-fluorescence output" display mechanism. Consequently, high-security 3D-encoding information carriers with an unprecedented combination of single-input multiple-output, dynamic/static dual-mode and spatially controlled display capacities are achieved. This bioinspired strategy brings functional-integrated features for artificial display systems and opens previously unidentified avenues for information security
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|a Journal Article
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|a bioinspired materials
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|a chemical‐gated actuation
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|a fluorescent patterning
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|a hydrogel
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|a information 3D‐encoding
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|a Si, Muqing
|e verfasserin
|4 aut
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|a Hua, Luqin
|e verfasserin
|4 aut
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|a Zhang, Dong
|e verfasserin
|4 aut
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|a Li, Wanning
|e verfasserin
|4 aut
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|a Zhao, Chuanzhuang
|e verfasserin
|4 aut
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|a Lu, Wei
|e verfasserin
|4 aut
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|a Chen, Tao
|e verfasserin
|4 aut
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 25 vom: 17. Juni, Seite e2401659
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:36
|g year:2024
|g number:25
|g day:17
|g month:06
|g pages:e2401659
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|u http://dx.doi.org/10.1002/adma.202401659
|3 Volltext
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|d 36
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