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240328s2024 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202308823
|2 doi
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|a pubmed24n1488.xml
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|a eng
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|a Wu, Xihu
|e verfasserin
|4 aut
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|a Stable n-Type Perylene Derivative Ladder Polymer with Antiambipolarity for Electrically Reconfigurable Organic Logic Gates
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|c 2024
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|a Text
|b txt
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|a ƒaComputermedien
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|2 rdamedia
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|a ƒa Online-Ressource
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|2 rdacarrier
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|a Date Revised 01.08.2024
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2024 Wiley‐VCH GmbH.
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|a Organic electrochemical transistors (OECTs) are one of the promising building blocks to realize next-generation bioelectronics. To date, however, the performance and signal processing capabilities of these devices remain limited by their stability and speed. Herein, the authors demonstrate stable and fast n-type organic electrochemical transistors based on a side-chain-free ladder polymer, poly(benzimidazoanthradiisoquinolinedione). The device demonstrated fast normalized transient speed of 0.56 ± 0.17 ms um-2 and excellent long-term stability in aqueous electrolytes, with no significant drop in its doping current after 50 000 successive doping/dedoping cycles and 2-month storage at ambient conditions. These unique characteristics make this polymer especially suitable for bioelectronics, such as being used as a pull-down channel in a complementary inverter for long-term stable detection of electrophysiological signals. Moreover, the developed device shows a reversible anti-ambipolar behavior, enabling reconfigurable electronics to be realized using a single material. These results go beyond the conventional OECT and demonstrate the potential of OECTs to exhibit dynamically configurable functionalities for next-generation reconfigurable electronics
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|a Journal Article
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|a n‐type
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|a antiambipolar
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|a electrically reconfigurable organic logic gates
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|a ladder‐type conjugated polymers
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|a organic electrochemical transistors
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|a stable
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|a He, Qiang
|e verfasserin
|4 aut
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|a Zhou, Zhongliang
|e verfasserin
|4 aut
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|a Tam, Teck Lip Dexter
|e verfasserin
|4 aut
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|a Tang, Cindy
|e verfasserin
|4 aut
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|a Lin, Ming
|e verfasserin
|4 aut
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|a Moser, Maximilian
|e verfasserin
|4 aut
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|a Griggs, Sophie
|e verfasserin
|4 aut
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|a Marks, Adam
|e verfasserin
|4 aut
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|a Chen, Shuai
|e verfasserin
|4 aut
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|a Xu, Jianwei
|e verfasserin
|4 aut
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|a McCulloch, Iain
|e verfasserin
|4 aut
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|a Leong, Wei Lin
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 31 vom: 01. Aug., Seite e2308823
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:36
|g year:2024
|g number:31
|g day:01
|g month:08
|g pages:e2308823
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|u http://dx.doi.org/10.1002/adma.202308823
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