Ternary BiOI/Bi2S3/Au Nanosheet Arrays as a Photoelectrochemical Signal Converter for the Detection of Cardiac Troponin I

Nanosheet arrays with stable signal output have become promising photoactive materials for photoelectrochemical (PEC) immunosensors. However, an essential concern is the facile recombination of carriers in one-component nanoarrays, which cannot be readily prevented, ultimately resulting in weak phot...

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Veröffentlicht in:Langmuir : the ACS journal of surfaces and colloids. - 1992. - 40(2024), 13 vom: 02. Apr., Seite 7060-7066
1. Verfasser: Xu, Weixuan (VerfasserIn)
Weitere Verfasser: Zhang, Xuelin, Liu, Shanghua, Jiang, Feng, Li, Yueyuan, Xu, Zhen, Li, Yueyun
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2024
Zugriff auf das übergeordnete Werk:Langmuir : the ACS journal of surfaces and colloids
Schlagworte:Journal Article Research Support, Non-U.S. Gov't Gold 7440-57-5 Troponin I Bismuth U015TT5I8H bismuth sulfide XZC47M60X8
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520 |a Nanosheet arrays with stable signal output have become promising photoactive materials for photoelectrochemical (PEC) immunosensors. However, an essential concern is the facile recombination of carriers in one-component nanoarrays, which cannot be readily prevented, ultimately resulting in weak photocurrent signals. In this study, an immunosensor using gold nanoparticle-anchored BiOI/Bi2S3 nanosheet arrays (BiOI/Bi2S3/Au) as a signal converter was fabricated for sensitive detection of cardiac troponin I (cTnI). The ternary nanosheet arrays were prepared by a simple method in which Bi2S3 was well-coated on the BiOI surface by in situ growth, whereas the addition of Au further improved the photoelectric conversion efficiency and could link more antibodies. The three-dimensional (3D) ordered sheet-like network array structure and BiOI/Bi2S3/Au ternary nanosheet arrays showed stable and high photoelectric signal output and no significant difference in signals across different batches under visible light excitation. The fabricated immunosensor has a sensitive response to the target detection marker cTnI in a wide linear range of 500 fg/mL to 50 ng/mL, and the detection limit was 32 fg/mL, demonstrating good stability and selectivity. This work not only shows the great application potential of ternary heterojunction arrays in the field of PEC immunosensors but also provides a useful exploration for improving the stability of immunosensors 
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650 4 |a Research Support, Non-U.S. Gov't 
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650 7 |a Troponin I  |2 NLM 
650 7 |a Bismuth  |2 NLM 
650 7 |a U015TT5I8H  |2 NLM 
650 7 |a bismuth sulfide  |2 NLM 
650 7 |a XZC47M60X8  |2 NLM 
700 1 |a Zhang, Xuelin  |e verfasserin  |4 aut 
700 1 |a Liu, Shanghua  |e verfasserin  |4 aut 
700 1 |a Jiang, Feng  |e verfasserin  |4 aut 
700 1 |a Li, Yueyuan  |e verfasserin  |4 aut 
700 1 |a Xu, Zhen  |e verfasserin  |4 aut 
700 1 |a Li, Yueyun  |e verfasserin  |4 aut 
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