Application of CuFeLDH-NCNT in ultrasound-assisted-Fenton-like process for removing ciprofloxacin from aqueous solutions
In this study, the mesoporous material NCNT was prepared by treating carbon nanotubes (CNT) with hydrazine and subsequently loaded with Cu-Fe layered double hydroxide (CuFeLDH) to create a multiphase catalyst (CuFeLDH-NCNT). Its application as a multiphase catalyst was investigated in an ultrasound-...
Veröffentlicht in: | Water science and technology : a journal of the International Association on Water Pollution Research. - 1986. - 89(2024), 5 vom: 14. März, Seite 1401-1417 |
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Weitere Verfasser: | , , , , |
Format: | Online-Aufsatz |
Sprache: | English |
Veröffentlicht: |
2024
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Zugriff auf das übergeordnete Werk: | Water science and technology : a journal of the International Association on Water Pollution Research |
Schlagworte: | Journal Article Hydrogen Peroxide BBX060AN9V Nanotubes, Carbon Ciprofloxacin 5E8K9I0O4U Hydroxides |
Zusammenfassung: | In this study, the mesoporous material NCNT was prepared by treating carbon nanotubes (CNT) with hydrazine and subsequently loaded with Cu-Fe layered double hydroxide (CuFeLDH) to create a multiphase catalyst (CuFeLDH-NCNT). Its application as a multiphase catalyst was investigated in an ultrasound-assisted Fenton process for ciprofloxacin (CIP) degradation in aqueous solution. In addition, the impacts of catalyst dosage, ultrasonic power, H2O2 dosage, and beginning pH on CIP removal efficiency were carefully evaluated to maximize the removal efficiency of CIP. The findings indicated that the elimination rate of the initial CIP concentration of 20 mg/L surpassed 94.66% after a mere 100 min, while the TOC degradation rate was 70.4%. The high removal rate was due to the synergistic action between the nanoparticles, H2O2, and ultrasonography. The degradation intermediates of CIP were examined, and putative degradation pathways and mechanisms were postulated |
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Beschreibung: | Date Completed 15.03.2024 Date Revised 15.03.2024 published: Print Citation Status MEDLINE |
ISSN: | 0273-1223 |
DOI: | 10.2166/wst.2024.066 |