Multi-Interfacial Confined Assembly of Colloidal Quantum Dots Quasisuperlattice Microcavities for High-Resolution Full-Color Microlaser Arrays

© 2024 Wiley‐VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 36(2024), 23 vom: 03. Juni, Seite e2314061
1. Verfasser: Li, Hui (VerfasserIn)
Weitere Verfasser: Zhao, Yuyan, Qiu, Yuchen, Gao, Hanfei, He, Ke, Yang, Junchuan, Zhao, Yingjie, OuYang, Guangwen, Ma, Na, Wei, Xiao, Du, Zuliang, Jiang, Lei, Wu, Yuchen
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2024
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article colloidal quantum dots full‐color laser arrays interface long‐range‐ordered assembly patterning
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520 |a Colloidal quantum dots (CQDs) are considered a promising material for the next generation of integrated display devices due to their designable optical bandgap and low energy consumption. Owing to their dispersibility in solvents, CQD micro/nanostructures are generally fabricated by solution-processing methods. However, the random mass transfer in liquid restricts the programmable construction in macroscopy and ordered assembly in microscopy for the integration of CQD optical structures. Herein, a multi-interfacial confined assembly strategy is developed to fabricate CQDs programmable microstructure arrays with a quasisuperlattice configuration through controlling the dynamics of three-phase contact lines (TPCLs). The motion of TPCLs dominates the division of liquid film for precise positioning of CQD microstructures, while pinned TPCLs control the solvent evaporation and concentration gradient to directionally drive the mass transfer and packing of CQDs. Owing to their long-range order and adjustable structural dimensions, CQD microring arrays function as high-quality-factor (high-Q) lasing resonant cavities with low thresholds and tunable lasing emission modes. Through the further surface treatment and liquid dynamics control, the on-chip integration of red (R), green (G), and blue (B) multicomponent CQD microlaser arrays are demonstrated. The technique establishes a new route to fabricate large-area, ultrahigh-definition, and full-color CQD laser displays 
650 4 |a Journal Article 
650 4 |a colloidal quantum dots 
650 4 |a full‐color laser arrays 
650 4 |a interface 
650 4 |a long‐range‐ordered assembly 
650 4 |a patterning 
700 1 |a Zhao, Yuyan  |e verfasserin  |4 aut 
700 1 |a Qiu, Yuchen  |e verfasserin  |4 aut 
700 1 |a Gao, Hanfei  |e verfasserin  |4 aut 
700 1 |a He, Ke  |e verfasserin  |4 aut 
700 1 |a Yang, Junchuan  |e verfasserin  |4 aut 
700 1 |a Zhao, Yingjie  |e verfasserin  |4 aut 
700 1 |a OuYang, Guangwen  |e verfasserin  |4 aut 
700 1 |a Ma, Na  |e verfasserin  |4 aut 
700 1 |a Wei, Xiao  |e verfasserin  |4 aut 
700 1 |a Du, Zuliang  |e verfasserin  |4 aut 
700 1 |a Jiang, Lei  |e verfasserin  |4 aut 
700 1 |a Wu, Yuchen  |e verfasserin  |4 aut 
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773 1 8 |g volume:36  |g year:2024  |g number:23  |g day:03  |g month:06  |g pages:e2314061 
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