Degradation of direct red 23 dye in a plug flow reactor with adjustable angle baffles using nano-Fe3O4 : modelling and optimisation

Photocatalytic degradation is a key technique in wastewater treatment, particularly for toxic dye removal, yet challenges related to poor hydrodynamics and mass transfer limitations persist. This study addresses these challenges by innovatively employing an adjustable-angle baffle in a plug flow rea...

Ausführliche Beschreibung

Bibliographische Detailangaben
Veröffentlicht in:Environmental technology. - 1993. - 45(2024), 27 vom: 01. Nov., Seite 5878-5898
1. Verfasser: Zoqi, Mohamad Javad (VerfasserIn)
Weitere Verfasser: Doosti, Mohamad Reza, Izadi, Sajad
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2024
Zugriff auf das übergeordnete Werk:Environmental technology
Schlagworte:Journal Article Baffle orientation azo dye genetic algorithm plug flow turbulence Water Pollutants, Chemical Coloring Agents Azo Compounds Wastewater
LEADER 01000caa a22002652c 4500
001 NLM36832723X
003 DE-627
005 20250305181458.0
007 cr uuu---uuuuu
008 240213s2024 xx |||||o 00| ||eng c
024 7 |a 10.1080/09593330.2024.2310525  |2 doi 
028 5 2 |a pubmed25n1225.xml 
035 |a (DE-627)NLM36832723X 
035 |a (NLM)38295843 
040 |a DE-627  |b ger  |c DE-627  |e rakwb 
041 |a eng 
100 1 |a Zoqi, Mohamad Javad  |e verfasserin  |4 aut 
245 1 0 |a Degradation of direct red 23 dye in a plug flow reactor with adjustable angle baffles using nano-Fe3O4  |b modelling and optimisation 
264 1 |c 2024 
336 |a Text  |b txt  |2 rdacontent 
337 |a ƒaComputermedien  |b c  |2 rdamedia 
338 |a ƒa Online-Ressource  |b cr  |2 rdacarrier 
500 |a Date Completed 01.12.2024 
500 |a Date Revised 01.12.2024 
500 |a published: Print-Electronic 
500 |a Citation Status MEDLINE 
520 |a Photocatalytic degradation is a key technique in wastewater treatment, particularly for toxic dye removal, yet challenges related to poor hydrodynamics and mass transfer limitations persist. This study addresses these challenges by innovatively employing an adjustable-angle baffle in a plug flow reactor (PFR) to enhance dye removal efficiency. A lab-scale PFR with an adjustable baffle was utilised to assess the impact of various factors, including baffle angle, catalyst concentration, hydraulic retention time (HRT), pH, and initial dye concentration, on the removal of direct red 23 dye. The experimental design employed a central composite design (CCD), with subsequent data analysis using response surface methodology (RSM) and artificial neural network (ANN) models. The findings demonstrate that the adjustable baffle significantly impacts dye removal, achieving maximum efficiency at an optimal angle of 77.5 degrees. The ANN model outperformed the RSM model, with a higher determination coefficient (R2) of 0.994 compared to 0.928. Furthermore, RSM and genetic algorithms yielded closely aligned optimal conditions, validating their accuracy. The optimised conditions achieved a dye removal efficiency of 89.47%. Significantly, the study also identified degradation as the dominant mechanism over adsorption and highlighted the impressive stability of nano-Fe3O4 during the recycling process. Mineralisation analysis revealed the presence of lightweight organic residual molecules post-treatment. These outcomes demonstrate the effectiveness of adjustable baffles in PFRs, marking a significant advancement in wastewater treatment technologies and underscoring the critical role of baffle orientation and catalyst concentration in optimising dye removal processes 
650 4 |a Journal Article 
650 4 |a Baffle orientation 
650 4 |a azo dye 
650 4 |a genetic algorithm 
650 4 |a plug flow 
650 4 |a turbulence 
650 7 |a Water Pollutants, Chemical  |2 NLM 
650 7 |a Coloring Agents  |2 NLM 
650 7 |a Azo Compounds  |2 NLM 
650 7 |a Wastewater  |2 NLM 
700 1 |a Doosti, Mohamad Reza  |e verfasserin  |4 aut 
700 1 |a Izadi, Sajad  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Environmental technology  |d 1993  |g 45(2024), 27 vom: 01. Nov., Seite 5878-5898  |w (DE-627)NLM098202545  |x 1479-487X  |7 nnas 
773 1 8 |g volume:45  |g year:2024  |g number:27  |g day:01  |g month:11  |g pages:5878-5898 
856 4 0 |u http://dx.doi.org/10.1080/09593330.2024.2310525  |3 Volltext 
912 |a GBV_USEFLAG_A 
912 |a SYSFLAG_A 
912 |a GBV_NLM 
912 |a GBV_ILN_350 
951 |a AR 
952 |d 45  |j 2024  |e 27  |b 01  |c 11  |h 5878-5898