Near-Zero Energy Consumption Capacitors by Controlling Inhomogeneous Polarization Configuration

© 2024 Wiley‐VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 36(2024), 21 vom: 18. Mai, Seite e2313285
1. Verfasser: Chen, Liang (VerfasserIn)
Weitere Verfasser: Hu, Tengfei, Shi, Xiaoming, Yu, Huifen, Zhang, Hao, Wu, Jie, Fu, Zhengqian, Qi, He, Chen, Jun
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2024
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article ceramic capacitors energy storage inhomogeneous polarization configuration lead‐free relaxors near‐zero energy loss
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520 |a Taking into account the need for energy conservation, achieving near-zero energy loss, namely ultrahigh efficiency (η), in energy storage capacitors with large recoverable energy storage density (Wrec) plays an important role in applications, which is one of the major challenges in dielectric energy storage field. Here, guided by phase-field simulation, inhomogeneous polarization configuration with multiple symmetries and polarization magnitudes is controlled through aliovalent strongly polar double ion design to establish a strongly disordered state. A record-high η of ≈97.4% is realized in lead-free relaxors with a large Wrec of ≈8.6 J cm-3, which also give a giant Wrec of ≈11.6 J cm-3 with an ultrahigh η of ≈96.1% through high-energy ball milling, showing a breakthrough progress in ceramic capacitors with a maximum figure of merit of 330. This work demonstrates that controlling inhomogeneous polarization configuration is an effective avenue to develop new high-performance near-zero energy loss energy storage capacitors 
650 4 |a Journal Article 
650 4 |a ceramic capacitors 
650 4 |a energy storage 
650 4 |a inhomogeneous polarization configuration 
650 4 |a lead‐free relaxors 
650 4 |a near‐zero energy loss 
700 1 |a Hu, Tengfei  |e verfasserin  |4 aut 
700 1 |a Shi, Xiaoming  |e verfasserin  |4 aut 
700 1 |a Yu, Huifen  |e verfasserin  |4 aut 
700 1 |a Zhang, Hao  |e verfasserin  |4 aut 
700 1 |a Wu, Jie  |e verfasserin  |4 aut 
700 1 |a Fu, Zhengqian  |e verfasserin  |4 aut 
700 1 |a Qi, He  |e verfasserin  |4 aut 
700 1 |a Chen, Jun  |e verfasserin  |4 aut 
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773 1 8 |g volume:36  |g year:2024  |g number:21  |g day:18  |g month:05  |g pages:e2313285 
856 4 0 |u http://dx.doi.org/10.1002/adma.202313285  |3 Volltext 
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