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240208s2024 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202313930
|2 doi
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|a pubmed24n1403.xml
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|a (DE-627)NLM368151247
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|a (NLM)38325888
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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| 100 |
1 |
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|a Zhang, Longlong
|e verfasserin
|4 aut
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| 245 |
1 |
0 |
|a Electrochemically Exfoliated Graphene Additive-Free Inks for 3D Printing Customizable Monolithic Integrated Micro-Supercapacitors on a Large Scale
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|c 2024
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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| 338 |
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|a ƒa Online-Ressource
|b cr
|2 rdacarrier
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|a Date Revised 09.05.2024
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2024 Wiley‐VCH GmbH.
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|a Three-dimensional (3D) printing technology with enhanced fidelity can achieve multiple functionalities and boost electrochemical performance of customizable planar micro-supercapacitors (MSCs), however, precise structural control of additive-free graphene-based macro-assembly electrode for monolithic integrated MSCs (MIMSCs) remains challenging. Here, the large-scale 3D printing fabrication of customizable planar MIMSCs is reported utilizing additive-free, high-quality electrochemically exfoliated graphene inks, which is not required the conventional cryogenic assistance during the printing process and any post-processing reduction. The resulting MSCs reveal an extremely small engineering footprint of 0.025 cm2, exceptionally high areal capacitance of 4900 mF cm-2, volumetric capacitance of 195.6 F cm-3, areal energy density of 2.1 mWh cm-2, and unprecedented volumetric energy density of 23 mWh cm-3 for a single cell, surpassing most previously reported 3D printed MSCs. The 3D printed MIMSC pack is further demonstrated, with the maximum areal cell count density of 16 cell cm-2, the highest output voltage of 192.5 V and the largest output voltage per unit area of 56 V cm-2 up to date are achieved. This work presents an innovative solution for processing high-performance additive-free graphene ink and realizing the large-scale production of 3D printed MIMSCs for planar energy storage
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4 |
|a Journal Article
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4 |
|a 3D printing
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| 650 |
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4 |
|a additive‐free
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| 650 |
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4 |
|a graphene ink
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| 650 |
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4 |
|a micro‐supercapacitors
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| 650 |
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4 |
|a monolithic integration
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| 700 |
1 |
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|a Qin, Jieqiong
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Das, Pratteek
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Wang, Sen
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Bai, Tiesheng
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Zhou, Feng
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Wu, Mingbo
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Wu, Zhong-Shuai
|e verfasserin
|4 aut
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| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 19 vom: 09. Mai, Seite e2313930
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
1 |
8 |
|g volume:36
|g year:2024
|g number:19
|g day:09
|g month:05
|g pages:e2313930
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| 856 |
4 |
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|u http://dx.doi.org/10.1002/adma.202313930
|3 Volltext
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