|
|
|
|
| LEADER |
01000caa a22002652 4500 |
| 001 |
NLM366509624 |
| 003 |
DE-627 |
| 005 |
20240405233333.0 |
| 007 |
cr uuu---uuuuu |
| 008 |
240108s2024 xx |||||o 00| ||eng c |
| 024 |
7 |
|
|a 10.1002/adma.202309183
|2 doi
|
| 028 |
5 |
2 |
|a pubmed24n1366.xml
|
| 035 |
|
|
|a (DE-627)NLM366509624
|
| 035 |
|
|
|a (NLM)38160321
|
| 040 |
|
|
|a DE-627
|b ger
|c DE-627
|e rakwb
|
| 041 |
|
|
|a eng
|
| 100 |
1 |
|
|a Kim, Jong Heon
|e verfasserin
|4 aut
|
| 245 |
1 |
0 |
|a Analogous Design of a Microlayered Silicon Oxide-Based Electrode to the General Electrode Structure for Thin-Film Lithium-Ion Batteries
|
| 264 |
|
1 |
|c 2024
|
| 336 |
|
|
|a Text
|b txt
|2 rdacontent
|
| 337 |
|
|
|a ƒaComputermedien
|b c
|2 rdamedia
|
| 338 |
|
|
|a ƒa Online-Ressource
|b cr
|2 rdacarrier
|
| 500 |
|
|
|a Date Revised 04.04.2024
|
| 500 |
|
|
|a published: Print-Electronic
|
| 500 |
|
|
|a Citation Status PubMed-not-MEDLINE
|
| 520 |
|
|
|a © 2024 Wiley‐VCH GmbH.
|
| 520 |
|
|
|a Development of miniaturized thin-film lithium-ion batteries (TF-LIBs) using vacuum deposition techniques is crucial for low-scale applications, but addressing low energy density remains a challenge. In this work, structures analogous to SiOx-based thin-film electrodes are designed with close resemblance to traditional LIB slurry formulations including active material, conductive agent, and binder. The thin-film is produced using mid-frequency sputtering with a single hybrid target consisting of SiOx nanoparticles, carbon nanotubes, and polytetrafluoroethylene. The thin-film SiOx/PPFC (plasma-polymerized fluorocarbon) involves a combination of SiOx and conductive carbon within the PPFC matrix. This results in enhanced electronic conductivity and superior elasticity and hardness in comparison to a conventional pure SiOx-based thin-film. The electrochemical performance of the half-cell consisting of thin-film SiOx/PPFC demonstrates remarkable cycling stability, with a capacity retention of 74.8% up to the 1000th cycle at 0.5 C. In addition, a full cell using the LiNi0.6Co0.2Mn0.2O2 thin-film as the cathode material exhibits an exceptional initial capacity of ≈120 mAh g-1 at 0.1 C and cycle performance, marked by a capacity retention of 90.8% from the first cycle to the 500th cycle at a 1 C rate. This work will be a stepping stone for the AM/CB/B composite electrodes in TF-LIBs
|
| 650 |
|
4 |
|a Journal Article
|
| 650 |
|
4 |
|a lithium‐ion batteries
|
| 650 |
|
4 |
|a polytetrafluoroethylene
|
| 650 |
|
4 |
|a silicon
|
| 650 |
|
4 |
|a sputtering
|
| 650 |
|
4 |
|a thin‐films
|
| 700 |
1 |
|
|a Song, Aeran
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Park, Ji-Min
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Park, Jun-Seob
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Behera, Subhashree
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Cho, Eunmi
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Park, Yun Chang
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Kim, Na-Yeong
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Jung, Ji-Won
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Lee, Sang-Jin
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Kim, Hyun-Suk
|e verfasserin
|4 aut
|
| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 14 vom: 05. Apr., Seite e2309183
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
|
| 773 |
1 |
8 |
|g volume:36
|g year:2024
|g number:14
|g day:05
|g month:04
|g pages:e2309183
|
| 856 |
4 |
0 |
|u http://dx.doi.org/10.1002/adma.202309183
|3 Volltext
|
| 912 |
|
|
|a GBV_USEFLAG_A
|
| 912 |
|
|
|a SYSFLAG_A
|
| 912 |
|
|
|a GBV_NLM
|
| 912 |
|
|
|a GBV_ILN_350
|
| 951 |
|
|
|a AR
|
| 952 |
|
|
|d 36
|j 2024
|e 14
|b 05
|c 04
|h e2309183
|