Preparation of composite coagulant for the removal of microplastics in water

© 2023 Water Environment Federation.

Bibliographische Detailangaben
Veröffentlicht in:Water environment research : a research publication of the Water Environment Federation. - 1998. - 95(2023), 12 vom: 01. Dez., Seite e10969
1. Verfasser: Sun, Yongjun (VerfasserIn)
Weitere Verfasser: Wu, Qu, Li, Xiaoqi, Sun, Wenquan, Zhou, Jun, Shah, Kinjal J
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2023
Zugriff auf das übergeordnete Werk:Water environment research : a research publication of the Water Environment Federation
Schlagworte:Journal Article composite flocculant flocculation flocculation mechanism micro-nano pollutant particle size analysis poly-N,N-dimethyl-N,N-diallylammonium chloride 26062-79-3 Wastewater Microplastics mehr... Plastics Titanium D1JT611TNE polyferric chloride
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245 1 0 |a Preparation of composite coagulant for the removal of microplastics in water 
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520 |a In this work, a composite flocculant (polyferric titanium sulfate-polydimethyldiallylammonium chloride [PFTS-PDMDAAC]) with a rich spatial network structure was prepared for the treatment of simulated wastewater containing polystyrene (PS) micro-nanoparticles. Characterization results showed that the surface of the PFTS-PDMDAAC was a three-dimensional network polymer of chain molecules that exhibited good thermal stability and formed an amorphous polymer containing multiply hydroxyl-bridged titanium and iron. When n(OH- ) : n(Fe) = 1:2, n(PO4 3- ) : n(Fe) = 0.35, n(Ti) : n(Fe) = 1:8, n(DMDAAC) : n(Fe) = 5:100, and the polymerization temperature is 60°C, the prepared composite flocculant has the best effect. The effects of dosage, pH, and agitation intensity on the flocculation properties of PFTS-PDMDAAC were also studied. The optimal removal rates of PS-μm and haze by PFTS-PDMDAAC were 85.60% and 90.10%, respectively, at a stirring intensity of 200 rpm, a pH of 9.0, and a PFTS-PDMDAAC dosage of 20 mg/L. The flocs produced by the PFTS-PDMDAAC flocculation were large and compact in structure, and the flocculation mechanism was mainly based on adsorption bridging. Kaolin played a promoting role in the process of PS-μm removal by PFTS-PDMDAAC floc and accelerated the formation of large and dense flocs. This study provided a reference for the coagulation method to remove micro-nanopollutants in the actual water treatment process. PRACTITIONER POINTS: A composite flocculant with rich spatial network structure (PFTS-PDMDAAC) was prepared. PFTS-PDMDAAC can effectively remove micro-nano polystyrene (PS) in wastewater. The floc produced by PFTS-PDMDAAC is large and compact in structure. The flocculation mechanism of PFTS-PDMDAAC is mainly adsorption bridging 
650 4 |a Journal Article 
650 4 |a composite flocculant 
650 4 |a flocculation 
650 4 |a flocculation mechanism 
650 4 |a micro-nano pollutant 
650 4 |a particle size analysis 
650 7 |a poly-N,N-dimethyl-N,N-diallylammonium chloride  |2 NLM 
650 7 |a 26062-79-3  |2 NLM 
650 7 |a Wastewater  |2 NLM 
650 7 |a Microplastics  |2 NLM 
650 7 |a Plastics  |2 NLM 
650 7 |a Titanium  |2 NLM 
650 7 |a D1JT611TNE  |2 NLM 
650 7 |a polyferric chloride  |2 NLM 
700 1 |a Wu, Qu  |e verfasserin  |4 aut 
700 1 |a Li, Xiaoqi  |e verfasserin  |4 aut 
700 1 |a Sun, Wenquan  |e verfasserin  |4 aut 
700 1 |a Zhou, Jun  |e verfasserin  |4 aut 
700 1 |a Shah, Kinjal J  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Water environment research : a research publication of the Water Environment Federation  |d 1998  |g 95(2023), 12 vom: 01. Dez., Seite e10969  |w (DE-627)NLM098214292  |x 1554-7531  |7 nnas 
773 1 8 |g volume:95  |g year:2023  |g number:12  |g day:01  |g month:12  |g pages:e10969 
856 4 0 |u http://dx.doi.org/10.1002/wer.10969  |3 Volltext 
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