Enhanced Adsorptive Removal of Tetracycline by Phosphomolybdic Acid-Modified Low-Temperature Sludge Biochar

Increasing the adsorption capacity and reducing the energy consumption of sludge biochar during preparation is important. In this study, a new modification method was developed to prepare phosphomolybdic acid-modified sludge biochar through the low-temperature pyrolysis of sewage sludge using phosph...

Ausführliche Beschreibung

Bibliographische Detailangaben
Veröffentlicht in:Langmuir : the ACS journal of surfaces and colloids. - 1992. - 40(2024), 1 vom: 09. Jan., Seite 751-760
1. Verfasser: Zhao, Liyang (VerfasserIn)
Weitere Verfasser: Li, Qian, Wang, Hengyi, Zhou, Zheng, Li, Nan, Pan, Honghui, Liu, Yan, Liu, Xixiang
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2024
Zugriff auf das übergeordnete Werk:Langmuir : the ACS journal of surfaces and colloids
Schlagworte:Journal Article Research Support, Non-U.S. Gov't Sewage phosphomolybdic acid RN225F04V1 biochar Anti-Bacterial Agents Tetracycline F8VB5M810T Charcoal mehr... 16291-96-6 Water Pollutants, Chemical
LEADER 01000caa a22002652 4500
001 NLM366003798
003 DE-627
005 20240215231951.0
007 cr uuu---uuuuu
008 231227s2024 xx |||||o 00| ||eng c
024 7 |a 10.1021/acs.langmuir.3c02973  |2 doi 
028 5 2 |a pubmed24n1294.xml 
035 |a (DE-627)NLM366003798 
035 |a (NLM)38109683 
040 |a DE-627  |b ger  |c DE-627  |e rakwb 
041 |a eng 
100 1 |a Zhao, Liyang  |e verfasserin  |4 aut 
245 1 0 |a Enhanced Adsorptive Removal of Tetracycline by Phosphomolybdic Acid-Modified Low-Temperature Sludge Biochar 
264 1 |c 2024 
336 |a Text  |b txt  |2 rdacontent 
337 |a ƒaComputermedien  |b c  |2 rdamedia 
338 |a ƒa Online-Ressource  |b cr  |2 rdacarrier 
500 |a Date Completed 11.01.2024 
500 |a Date Revised 15.02.2024 
500 |a published: Print-Electronic 
500 |a Citation Status MEDLINE 
520 |a Increasing the adsorption capacity and reducing the energy consumption of sludge biochar during preparation is important. In this study, a new modification method was developed to prepare phosphomolybdic acid-modified sludge biochar through the low-temperature pyrolysis of sewage sludge using phosphomolybdic acid as a modifier. Tetracycline was used to assess the adsorption performance of sludge biochar, and phosphomolybdic acid-modified sludge biochar was prepared at different temperatures. The results showed that the adsorption capacity of sludge biochar improved from 84.49 to 120.86 mg/g through modification with phosphomolybdic acid at 200 °C. The maximum adsorption capacities of phosphomolybdic acid-modified sludge biochar (200 °C pyrolysis temperature) at 298, 308, and 318 K were 283.87, 421.39, and 545.48 mg/g, respectively. Both liquid film and intraparticle diffusion were the main rate-limiting steps of tetracycline adsorption by phosphomolybdic acid-modified sludge biochar. Furthermore, the adsorption of tetracycline by phosphomolybdic acid-modified sludge biochar was mainly attributed to π-π interactions, electrostatic interactions, hydrogen bonding, and pore filling 
650 4 |a Journal Article 
650 4 |a Research Support, Non-U.S. Gov't 
650 7 |a Sewage  |2 NLM 
650 7 |a phosphomolybdic acid  |2 NLM 
650 7 |a RN225F04V1  |2 NLM 
650 7 |a biochar  |2 NLM 
650 7 |a Anti-Bacterial Agents  |2 NLM 
650 7 |a Tetracycline  |2 NLM 
650 7 |a F8VB5M810T  |2 NLM 
650 7 |a Charcoal  |2 NLM 
650 7 |a 16291-96-6  |2 NLM 
650 7 |a Water Pollutants, Chemical  |2 NLM 
700 1 |a Li, Qian  |e verfasserin  |4 aut 
700 1 |a Wang, Hengyi  |e verfasserin  |4 aut 
700 1 |a Zhou, Zheng  |e verfasserin  |4 aut 
700 1 |a Li, Nan  |e verfasserin  |4 aut 
700 1 |a Pan, Honghui  |e verfasserin  |4 aut 
700 1 |a Liu, Yan  |e verfasserin  |4 aut 
700 1 |a Liu, Xixiang  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Langmuir : the ACS journal of surfaces and colloids  |d 1992  |g 40(2024), 1 vom: 09. Jan., Seite 751-760  |w (DE-627)NLM098181009  |x 1520-5827  |7 nnns 
773 1 8 |g volume:40  |g year:2024  |g number:1  |g day:09  |g month:01  |g pages:751-760 
856 4 0 |u http://dx.doi.org/10.1021/acs.langmuir.3c02973  |3 Volltext 
912 |a GBV_USEFLAG_A 
912 |a SYSFLAG_A 
912 |a GBV_NLM 
912 |a GBV_ILN_22 
912 |a GBV_ILN_350 
912 |a GBV_ILN_721 
951 |a AR 
952 |d 40  |j 2024  |e 1  |b 09  |c 01  |h 751-760