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231227s2024 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202307280
|2 doi
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|a pubmed24n1328.xml
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|a DE-627
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|a eng
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|a Zheng, Xiangjun
|e verfasserin
|4 aut
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|a Thorough Optimization for Intrinsically Stretchable Organic Photovoltaics
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|c 2024
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|a Text
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|a ƒaComputermedien
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|a ƒa Online-Ressource
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|a Date Revised 14.03.2024
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2023 Wiley-VCH GmbH.
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|a The development of intrinsically stretchable organic photovoltaics (is-OPVs) with a high efficiency is of significance for practical application. However, their efficiencies lag far behind those of rigid or even flexible counterparts. To address this issue, an advanced top-illuminated OPV is designed and fabricated, which is intrinsically stretchable and has a high performance, through systematic optimizations from material to device. First, the stretchability of the active layer is largely increased by adding a low-elastic-modulus elastomer of styrene-ethylene-propylene-styrene tri-block copolymer (SEPS). Second, the stretchability and conductivity of the opaque electrode are enhanced by a conductive polymer/metal (denoted as M-PH1000Ag) composite electrode strategy. Third, the optical and electrical properties of a sliver nanowire transparent electrode are improved by a solvent vapor annealing strategy. High-performance is-OPVs are successfully fabricated with a top-illuminated structure, which provides a record-high efficiency of 16.23%. Additionally, by incorporating 5-10% elastomer, a balance between the efficiency and stretchability of the is-OPVs is achieved. This study provides valuable insights into material and device optimizations for high-efficiency is-OPVs, with a low-cost production and excellent stretchability, which indicates a high potential for future applications of OPVs
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|a Journal Article
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|a AgNWs transparent electrode
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|a ITO-free devices
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|a composite electrode
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|a stretchable organic photovoltaics
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|a top-illuminated devices
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|a Wu, Xiaoling
|e verfasserin
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|a Wu, Qiang
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|a Han, Yunfei
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|a Ding, Guanyu
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|a Wang, Yiming
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|a Kong, Yibo
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|a Chen, Tianyi
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|a Wang, Mengting
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|a Zhang, Yiqing
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|a Xue, Jingwei
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|a Fu, Weifei
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|a Luo, Qun
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|a Ma, Changqi
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|a Ma, Wei
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|a Zuo, Lijian
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|a Shi, Minmin
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|a Chen, Hongzheng
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 11 vom: 01. März, Seite e2307280
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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|g volume:36
|g year:2024
|g number:11
|g day:01
|g month:03
|g pages:e2307280
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|u http://dx.doi.org/10.1002/adma.202307280
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