Tailoring Graphite into Subnanometer Graphene

© 2024 Wiley‐VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 36(2024), 15 vom: 10. Apr., Seite e2310022
1. Verfasser: Chen, Zhexue (VerfasserIn)
Weitere Verfasser: Zhang, Yutong, Zhao, Ce, Xia, Yuexing, Li, Zhangqiang, Zhou, Xuanping, Xiao, Liuyang, Liu, Xinfeng, Zhang, Yong
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2024
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article broken lattice graphene nonlinear saturation absorption photoluminescence sub‐1 nm
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520 |a Within the intersection of materials science and nanoscience/technology, extremely downsized (including quantum-sized and subnanometer-sized) materials attract increasing interest. However, the effective and controllable production of extremely downsized materials through physical strategies remains a great challenge. Herein, an all-physical top-down method for the production of sub-1 nm graphene with completely broken lattice is reported. The graphene subnanometer materials (GSNs) with monolayer structures and lateral sizes of ≈0.5 nm are obtained. Compared with their bulk, nanosheets, and quantum sheets, the intrinsic GSNs present extremely enhanced photoluminescence and nonlinear saturation absorption performances, as well as unique carrier behavior. The non-equilibrium states induced by the entirely exposed and broken, intrinsic lattices in sub-1 nm graphene can be determinative to their extreme performances. This work shows the great potential of broken lattice and provides new insights toward subnanometer materials 
650 4 |a Journal Article 
650 4 |a broken lattice 
650 4 |a graphene 
650 4 |a nonlinear saturation absorption 
650 4 |a photoluminescence 
650 4 |a sub‐1 nm 
700 1 |a Zhang, Yutong  |e verfasserin  |4 aut 
700 1 |a Zhao, Ce  |e verfasserin  |4 aut 
700 1 |a Xia, Yuexing  |e verfasserin  |4 aut 
700 1 |a Li, Zhangqiang  |e verfasserin  |4 aut 
700 1 |a Zhou, Xuanping  |e verfasserin  |4 aut 
700 1 |a Xiao, Liuyang  |e verfasserin  |4 aut 
700 1 |a Liu, Xinfeng  |e verfasserin  |4 aut 
700 1 |a Zhang, Yong  |e verfasserin  |4 aut 
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773 1 8 |g volume:36  |g year:2024  |g number:15  |g day:10  |g month:04  |g pages:e2310022 
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