An Antidehydration Hydrogel Based on Zwitterionic Oligomers for Bioelectronic Interfacing

© 2023 Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 36(2024), 8 vom: 01. Feb., Seite e2311255
1. Verfasser: He, Ke (VerfasserIn)
Weitere Verfasser: Cai, Pingqiang, Ji, Shaobo, Tang, Zihan, Fang, Zhou, Li, Wenlong, Yu, Jing, Su, Jiangtao, Luo, Yifei, Zhang, Feilong, Wang, Ting, Wang, Ming, Wan, Changjin, Pan, Liang, Ji, Baohua, Li, Dechang, Chen, Xiaodong
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2024
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article antidehydration bioelectronic interface hydrogel skin safety zwitterionic oligomer Hydrogels Salts
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520 |a Hydrogels are ideal interfacing materials for on-skin healthcare devices, yet their susceptibility to dehydration hinders their practical use. While incorporating hygroscopic metal salts can prevent dehydration and maintain ionic conductivity, concerns arise regarding metal toxicity due to the passage of small ions through the skin barrier. Herein, an antidehydration hydrogel enabled by the incorporation of zwitterionic oligomers into its network is reported. This hydrogel exhibits exceptional water retention properties, maintaining ≈88% of its weight at 40% relative humidity, 25 °C for 50 days and about 84% after being heated at 50 °C for 3 h. Crucially, the molecular weight design of the embedded oligomers prevents their penetration into the epidermis, as evidenced by experimental and molecular simulation results. The hydrogel allows stable signal acquisition in electrophysiological monitoring of humans and plants under low-humidity conditions. This research provides a promising strategy for the development of epidermis-safe and biocompatible antidehydration hydrogel interfaces for on-skin devices 
650 4 |a Journal Article 
650 4 |a antidehydration 
650 4 |a bioelectronic interface 
650 4 |a hydrogel 
650 4 |a skin safety 
650 4 |a zwitterionic oligomer 
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650 7 |a Salts  |2 NLM 
700 1 |a Cai, Pingqiang  |e verfasserin  |4 aut 
700 1 |a Ji, Shaobo  |e verfasserin  |4 aut 
700 1 |a Tang, Zihan  |e verfasserin  |4 aut 
700 1 |a Fang, Zhou  |e verfasserin  |4 aut 
700 1 |a Li, Wenlong  |e verfasserin  |4 aut 
700 1 |a Yu, Jing  |e verfasserin  |4 aut 
700 1 |a Su, Jiangtao  |e verfasserin  |4 aut 
700 1 |a Luo, Yifei  |e verfasserin  |4 aut 
700 1 |a Zhang, Feilong  |e verfasserin  |4 aut 
700 1 |a Wang, Ting  |e verfasserin  |4 aut 
700 1 |a Wang, Ming  |e verfasserin  |4 aut 
700 1 |a Wan, Changjin  |e verfasserin  |4 aut 
700 1 |a Pan, Liang  |e verfasserin  |4 aut 
700 1 |a Ji, Baohua  |e verfasserin  |4 aut 
700 1 |a Li, Dechang  |e verfasserin  |4 aut 
700 1 |a Chen, Xiaodong  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Advanced materials (Deerfield Beach, Fla.)  |d 1998  |g 36(2024), 8 vom: 01. Feb., Seite e2311255  |w (DE-627)NLM098206397  |x 1521-4095  |7 nnns 
773 1 8 |g volume:36  |g year:2024  |g number:8  |g day:01  |g month:02  |g pages:e2311255 
856 4 0 |u http://dx.doi.org/10.1002/adma.202311255  |3 Volltext 
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