UV-Curing Assisted Direct Ink Writing of Dense, Crack-Free, and High-Performance Zirconia-Based Composites With Aligned Alumina Platelets

© 2023 Wiley-VCH GmbH.

Détails bibliographiques
Publié dans:Advanced materials (Deerfield Beach, Fla.). - 1998. - 36(2024), 5 vom: 14. Feb., Seite e2306764
Auteur principal: Li, Maoyin (Auteur)
Autres auteurs: Huang, Shuigen, Willems, Evita, Soete, Jeroen, Inokoshi, Masanao, Van Meerbeek, Bart, Vleugels, Jef, Zhang, Fei
Format: Article en ligne
Langue:English
Publié: 2024
Accès à la collection:Advanced materials (Deerfield Beach, Fla.)
Sujets:Journal Article UV-curing direct ink writing laminate structures mechanical properties non-reactive diluent platelet alignment zirconia ceramics
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520 |a Additive manufacturing (AM) of high-performance structural ceramic components with comparative strength and toughness as conventionally manufactured ceramics remains challenging. Here, a UV-curing approach is integrated in direct ink writing (DIW), taking advantage from DIW to enable an easy use of high solid-loading pastes and multi-layered materials with compositional changes; while, avoiding drying problems. UV-curable opaque zirconia-based slurries with a solid loading of 51 vol% are developed to fabricate dense and crack-free alumina-toughened zirconia (ATZ) containing 3 wt% alumina platelets. Importantly, a non-reactive diluent is added to relieve polymerization-induced internal stresses, avoid subsequent warping and cracking, and facilitate the de-binding. For the first time, UV-curing assisted DIW-printed ceramic after sintering reveals even better mechanical properties than that processed by a conventional pressing. This is attributed to the aligned alumina platelets, enhancing crack deflection and improving the fracture toughness from 6.8 ± 0.3 MPa m0.5 (compacted) to 7.4 ± 0.3 MPa m0.5 (DIW). The four-point bending strength of the DIW ATZ (1009 ± 93 MPa) is also higher than that of the conventionally manufactured equivalent (861 ± 68 MPa). Besides homogeneous ceramic, laminate structures are demonstrated. This work provides a valuable hybrid approach to additively manufacture tough and strong ceramic components 
650 4 |a Journal Article 
650 4 |a UV-curing 
650 4 |a direct ink writing 
650 4 |a laminate structures 
650 4 |a mechanical properties 
650 4 |a non-reactive diluent 
650 4 |a platelet alignment 
650 4 |a zirconia ceramics 
700 1 |a Huang, Shuigen  |e verfasserin  |4 aut 
700 1 |a Willems, Evita  |e verfasserin  |4 aut 
700 1 |a Soete, Jeroen  |e verfasserin  |4 aut 
700 1 |a Inokoshi, Masanao  |e verfasserin  |4 aut 
700 1 |a Van Meerbeek, Bart  |e verfasserin  |4 aut 
700 1 |a Vleugels, Jef  |e verfasserin  |4 aut 
700 1 |a Zhang, Fei  |e verfasserin  |4 aut 
773 0 8 |i Enthalten in  |t Advanced materials (Deerfield Beach, Fla.)  |d 1998  |g 36(2024), 5 vom: 14. Feb., Seite e2306764  |w (DE-627)NLM098206397  |x 1521-4095  |7 nnas 
773 1 8 |g volume:36  |g year:2024  |g number:5  |g day:14  |g month:02  |g pages:e2306764 
856 4 0 |u http://dx.doi.org/10.1002/adma.202306764  |3 Volltext 
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