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231226s2024 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202309753
|2 doi
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|a pubmed25n1213.xml
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|a DE-627
|b ger
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|a eng
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| 100 |
1 |
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|a Lu, Hongyu
|e verfasserin
|4 aut
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| 245 |
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|a Microfluidic-Assisted 3D Printing Zinc Powder Anode with 2D Conductive MOF/MXene Heterostructures for High-Stable Zinc-Organic Battery
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|c 2024
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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|a ƒa Online-Ressource
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|a Date Revised 08.02.2024
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2023 Wiley-VCH GmbH.
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|a Zinc powder (Zn-P) anodes have significant advantages in terms of universality and machinability compared with Zn foil anodes. However, their rough surface, which has a high surface area, intensifies the uncontrollable growth of Zn dendrites and parasitic side reactions. In this study, an anti-corrosive Zn-P-based anode with a functional layer formed from a MXene and Cu-THBQ (MXene/Cu-THBQ) heterostructure is successfully fabricated via microfluidic-assisted 3D printing. The unusual anti-corrosive and strong adsorption of Zn ions using the MXene/Cu-THBQ functional layer can effectively homogenize the Zn ion flux and inhibit the hydrogen evolution reaction (HER) during the repeated process of Zn plating/stripping, thus achieving stable Zn cycling. Consequently, a symmetric cell based on Zn-P with the MXene/Cu-THBQ anode exhibits a highly reversible cycling of 1800 h at 2 mA cm-2 /1 mAh cm-2 . Furthermore, a Zn-organic full battery matched with a 4-hydroxy-2,2,6,6-tetramethylpiperidine-1-oxyl organic cathode riveted on graphene delivers a high reversible capacity and maintains a long cycle life
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|a Journal Article
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|a 2D conductive metal-organic frameworks
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4 |
|a 2D heterostructures
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4 |
|a MXenes
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4 |
|a zinc powder anodes
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| 650 |
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4 |
|a zinc-organic batteries
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| 700 |
1 |
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|a Hu, Jisong
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Zhang, Kaiqi
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Zhao, Jingxin
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Deng, Shenzhen
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Li, Yujie
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Xu, Bingang
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Pang, Huan
|e verfasserin
|4 aut
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| 773 |
0 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 6 vom: 04. Feb., Seite e2309753
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnas
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| 773 |
1 |
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|g volume:36
|g year:2024
|g number:6
|g day:04
|g month:02
|g pages:e2309753
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|u http://dx.doi.org/10.1002/adma.202309753
|3 Volltext
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