Scaling-Up Insights for Zinc-Air Battery Technologies Realizing Reversible Zinc Anodes

© 2023 The Authors. Advanced Materials published by Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 35(2023), 48 vom: 26. Nov., Seite e2303509
1. Verfasser: Shinde, Sambhaji S (VerfasserIn)
Weitere Verfasser: Wagh, Nayantara K, Lee, Chi Ho, Kim, Dong-Hyung, Kim, Sung-Hae, Um, Han-Don, Lee, Sang Uck, Lee, Jung-Ho
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2023
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article cell-level energy metrics pouch cell configurations principal testing parameters reversible Zn anodes thermodynamics and chemical kinetics
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520 |a Zinc-air battery (ZAB) technology is considered one of the promising candidates to complement the existing lithium-ion batteries for future large-scale high-energy-storage demands. The scientific literature reveals many efforts for the ZAB chemistries, materials design, and limited accounts for cell design principles with apparently superior performances for liquid and solid-state electrolytes. However, along with the difficulty of forming robust solid-electrolyte interphases, the discrepancy in testing methods and assessment metrics severely challenges the realistic evaluation/comparison and commercialization of ZABs. Here, strategies to formulate reversible zinc anodes are proposed and specific cell-level energy metrics (100-500 Wh kg-1 ) and realistic long-cycling operations are realized. Stabilizing anode/electrolyte interfaces results in a cumulative capacity of 25 Ah cm-2 and Coulomb efficiency of >99.9% for 5000 plating/stripping cycles. Using 1-10 Ah scale (≈500 Wh kg-1 at cell level) solid-state zinc-air pouch cells, scale-up insights for Ah-level ZABs that can progress from lab-scale research to practical production are also offered 
650 4 |a Journal Article 
650 4 |a cell-level energy metrics 
650 4 |a pouch cell configurations 
650 4 |a principal testing parameters 
650 4 |a reversible Zn anodes 
650 4 |a thermodynamics and chemical kinetics 
700 1 |a Wagh, Nayantara K  |e verfasserin  |4 aut 
700 1 |a Lee, Chi Ho  |e verfasserin  |4 aut 
700 1 |a Kim, Dong-Hyung  |e verfasserin  |4 aut 
700 1 |a Kim, Sung-Hae  |e verfasserin  |4 aut 
700 1 |a Um, Han-Don  |e verfasserin  |4 aut 
700 1 |a Lee, Sang Uck  |e verfasserin  |4 aut 
700 1 |a Lee, Jung-Ho  |e verfasserin  |4 aut 
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773 1 8 |g volume:35  |g year:2023  |g number:48  |g day:26  |g month:11  |g pages:e2303509 
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