|
|
|
|
| LEADER |
01000caa a22002652 4500 |
| 001 |
NLM362156786 |
| 003 |
DE-627 |
| 005 |
20240114233747.0 |
| 007 |
cr uuu---uuuuu |
| 008 |
231226s2024 xx |||||o 00| ||eng c |
| 024 |
7 |
|
|a 10.1002/adma.202304225
|2 doi
|
| 028 |
5 |
2 |
|a pubmed24n1256.xml
|
| 035 |
|
|
|a (DE-627)NLM362156786
|
| 035 |
|
|
|a (NLM)37718710
|
| 040 |
|
|
|a DE-627
|b ger
|c DE-627
|e rakwb
|
| 041 |
|
|
|a eng
|
| 100 |
1 |
|
|a Wei, Yanan
|e verfasserin
|4 aut
|
| 245 |
1 |
0 |
|a Over 18% Efficiency Ternary Organic Solar Cells with 300 nm Thick Active Layer Enabled by an Oligomeric Acceptor
|
| 264 |
|
1 |
|c 2024
|
| 336 |
|
|
|a Text
|b txt
|2 rdacontent
|
| 337 |
|
|
|a ƒaComputermedien
|b c
|2 rdamedia
|
| 338 |
|
|
|a ƒa Online-Ressource
|b cr
|2 rdacarrier
|
| 500 |
|
|
|a Date Revised 11.01.2024
|
| 500 |
|
|
|a published: Print-Electronic
|
| 500 |
|
|
|a Citation Status PubMed-not-MEDLINE
|
| 520 |
|
|
|a © 2023 Wiley-VCH GmbH.
|
| 520 |
|
|
|a The development of high-efficiency thickness-insensitive organic solar cells (OSCs) is crucially important for the mass production of solar panels. However, increasing the active layer thickness usually induces a substantial loss in efficiency. Herein, a ternary strategy in which an oligomer DY-TF is incorporated into PM6:L8-BO system as a guest component is adopted to break this dilemma. The S···F intramolecular noncovalent interactions in the backbone endow DY-TF with a high planarity. Upon the addition of DY-TF, the crystallinity of the blend is effectively improved, leading to increased charge carrier mobility, which is highly desirable in the fabrication of thick-film devices. As a result, thin-film PM6:L8-BO:DY-TF-based device (110 nm) shows a power conversion efficiency (PCE) of 19.13%. Impressively, when the active layer thickness increases to 300 nm, an efficiency of 18.23% (certified as 17.8%) is achieved, representing the highest efficiency reported for 300 nm thick OSCs thus far. Additionally, blade-coated thick device (300 nm) delivers a promising PCE of 17.38%. This work brings new insights into the construction of efficient OSCs with high thickness tolerance, showing great potential for roll-to-roll printing of large-area solar cells
|
| 650 |
|
4 |
|a Journal Article
|
| 650 |
|
4 |
|a efficiency
|
| 650 |
|
4 |
|a oligomer
|
| 650 |
|
4 |
|a organic solar cells
|
| 650 |
|
4 |
|a ternary blend
|
| 650 |
|
4 |
|a thickness tolerance
|
| 700 |
1 |
|
|a Cai, Yunhao
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Gu, Xiaobin
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Yao, Guo
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Fu, Zhen
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Zhu, Yuxuan
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Yang, Junfang
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Dai, Junpeng
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Zhang, Jianqi
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Zhang, Xin
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Hao, Xiaotao
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Lu, Guanghao
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Tang, Zheng
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Peng, Qian
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Zhang, Chunfeng
|e verfasserin
|4 aut
|
| 700 |
1 |
|
|a Huang, Hui
|e verfasserin
|4 aut
|
| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 36(2024), 2 vom: 08. Jan., Seite e2304225
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
|
| 773 |
1 |
8 |
|g volume:36
|g year:2024
|g number:2
|g day:08
|g month:01
|g pages:e2304225
|
| 856 |
4 |
0 |
|u http://dx.doi.org/10.1002/adma.202304225
|3 Volltext
|
| 912 |
|
|
|a GBV_USEFLAG_A
|
| 912 |
|
|
|a SYSFLAG_A
|
| 912 |
|
|
|a GBV_NLM
|
| 912 |
|
|
|a GBV_ILN_350
|
| 951 |
|
|
|a AR
|
| 952 |
|
|
|d 36
|j 2024
|e 2
|b 08
|c 01
|h e2304225
|