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231226s2023 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202303993
|2 doi
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|a pubmed24n1202.xml
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|a eng
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|a Patrian, Marta
|e verfasserin
|4 aut
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|a Genetically Encoded Oligomerization for Protein-Based Lighting Devices
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|c 2023
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|a Text
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|a ƒaComputermedien
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|a ƒa Online-Ressource
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|a Date Completed 29.11.2023
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|a Date Revised 29.11.2023
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|a published: Print-Electronic
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|a Citation Status MEDLINE
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|a © 2023 The Authors. Advanced Materials published by Wiley-VCH GmbH.
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|a Implementing proteins in optoelectronics represents a fresh idea toward a sustainable new class of materials with bio-functions that can replace environmentally unfriendly and/or toxic components without losing device performance. However, their native activity (fluorescence, catalysis, and so on) is easily lost under device fabrication/operation as non-native environments (organic solvents, organic/inorganic interfaces, and so on) and severe stress (temperature, irradiation, and so on) are involved. Herein, a gift bow genetically-encoded macro-oligomerization strategy is showcased to promote protein-protein solid interaction enabling i) high versatility with arbitrary proteins, ii) straightforward electrostatic driven control of the macro-oligomer size by ionic strength, and iii) stabilities over months in pure organic solvents and stress scenarios, allowing to integrate them into classical water-free polymer-based materials/components for optoelectronics. Indeed, rainbow-/white-emitting protein-based light-emitting diodes are fabricated, attesting a first-class performance compared to those with their respective native proteins: significantly enhanced device stabilities from a few minutes up to 100 h keeping device efficiency at high power driving conditions. Thus, the oligomerization concept is a solid bridge between biological systems and materials/components to meet expectations in bio-optoelectronics, in general, and lighting schemes, in particular
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|a Journal Article
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|a bio-hybrid light-emitting diodes
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|a engineered fluorescent proteins
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|a oligomerization
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|a organic solvent stability
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|a protein-based lighting
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|a Polymers
|2 NLM
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|a Solvents
|2 NLM
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|a Nieddu, Mattia
|e verfasserin
|4 aut
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|a Banda-Vázquez, Jesús A
|e verfasserin
|4 aut
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|a Gutierrez-Armayor, David
|e verfasserin
|4 aut
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|a González-Gaitano, Gustavo
|e verfasserin
|4 aut
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|a Fuenzalida-Werner, Juan Pablo
|e verfasserin
|4 aut
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|a Costa, Rubén D
|e verfasserin
|4 aut
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| 773 |
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|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 35(2023), 48 vom: 02. Nov., Seite e2303993
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|x 1521-4095
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|g volume:35
|g year:2023
|g number:48
|g day:02
|g month:11
|g pages:e2303993
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|u http://dx.doi.org/10.1002/adma.202303993
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