Toward Chiral Lasing from All-Solution-Processed Flexible Perovskite-Nanocrystal-Liquid-Crystal Membranes

© 2023 Wiley-VCH GmbH.

Bibliographische Detailangaben
Veröffentlicht in:Advanced materials (Deerfield Beach, Fla.). - 1998. - 35(2023), 44 vom: 02. Nov., Seite e2301573
1. Verfasser: Lin, Weixi (VerfasserIn)
Weitere Verfasser: Yang, Chao, Miao, Yu, Li, Sen, Zhang, Limin, Jiang, Xiao-Fang, Lv, Ying, Poudel, Bed, Wang, Kai, Polavarapu, Lakshminarayana, Zhang, Chen, Zhou, Guofu, Hu, Xiaowen
Format: Online-Aufsatz
Sprache:English
Veröffentlicht: 2023
Zugriff auf das übergeordnete Werk:Advanced materials (Deerfield Beach, Fla.)
Schlagworte:Journal Article circularly polarized lasing flexible membrane laser liquid crystals perovskite nanocrystals
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520 |a Circularly polarized (CP) coherent light sources are of great potential for various advanced optical applications spanning displays/imaging to data processing/encryption and quantum communication. Here, the first demonstration of CP amplified spontaneous emission (ASE)/lasing from a free-standing and flexible membrane device is reported. The membrane device consists of perovskite nanocrystals (PNCs) and cholesteric liquid crystals (CLCs) layers sandwiched within a Fabry-Pérot (F-P) cavity architecture. The chiral liquid crystal cavity enables the generation of CP light from the device. The device is completely solution-processable and displays CP ASE with record dissymmetry factor (glum ) as high as 1.4, which is 3 orders of magnitude higher as compared with glum of CP luminescence of chiral ligand-capped colloidal PNCs. The device exhibits ultraflexibility as the ASE intensity remains unchanged after repeated 100 bending cycles and it is stable for more than 3 months with 80% of its original intensity. Furthermore, the ultraflexibility enables the generation of ASE from various objects of different geometric surfaces covered with the flexible perovskite membrane device. This work not only demonstrates the first CP ASE from a PNCs membrane with extremely high glum but also opens the door toward the fabrication of ultraflexible, extremely stable, and all solution-processable perovskite chiral laser devices 
650 4 |a Journal Article 
650 4 |a circularly polarized lasing 
650 4 |a flexible membrane 
650 4 |a laser 
650 4 |a liquid crystals 
650 4 |a perovskite nanocrystals 
700 1 |a Yang, Chao  |e verfasserin  |4 aut 
700 1 |a Miao, Yu  |e verfasserin  |4 aut 
700 1 |a Li, Sen  |e verfasserin  |4 aut 
700 1 |a Zhang, Limin  |e verfasserin  |4 aut 
700 1 |a Jiang, Xiao-Fang  |e verfasserin  |4 aut 
700 1 |a Lv, Ying  |e verfasserin  |4 aut 
700 1 |a Poudel, Bed  |e verfasserin  |4 aut 
700 1 |a Wang, Kai  |e verfasserin  |4 aut 
700 1 |a Polavarapu, Lakshminarayana  |e verfasserin  |4 aut 
700 1 |a Zhang, Chen  |e verfasserin  |4 aut 
700 1 |a Zhou, Guofu  |e verfasserin  |4 aut 
700 1 |a Hu, Xiaowen  |e verfasserin  |4 aut 
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773 1 8 |g volume:35  |g year:2023  |g number:44  |g day:02  |g month:11  |g pages:e2301573 
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