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231226s2023 xx |||||o 00| ||eng c |
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|a 10.1002/adma.202305368
|2 doi
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|a pubmed24n1198.xml
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|a (DE-627)NLM359598986
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|a (NLM)37459236
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|a DE-627
|b ger
|c DE-627
|e rakwb
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|a eng
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| 100 |
1 |
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|a Wang, Mingming
|e verfasserin
|4 aut
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| 245 |
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|a Anions Regulation Engineering Enables a Highly Reversible and Dendrite-Free Nickel-Metal Anode with Ultrahigh Capacities
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|c 2023
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|a Text
|b txt
|2 rdacontent
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|a ƒaComputermedien
|b c
|2 rdamedia
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| 338 |
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|a ƒa Online-Ressource
|b cr
|2 rdacarrier
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|a Date Revised 20.10.2023
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|a published: Print-Electronic
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|a Citation Status PubMed-not-MEDLINE
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|a © 2023 Wiley-VCH GmbH.
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|a The development of safe and high-energy metal anodes represents a crucial research direction. Here, the achievement of highly reversible, dendrite-free transition metal anodes with ultrahigh capacities by regulating aqueous electrolytes is reported. Using nickel (Ni) as a model, theoretical and experimental evidence demonstrating the beneficial role of chloride ions in inhibiting and disrupting the nickel hydroxide passivation layer on the Ni electrode is provided. As a result, Ni anodes with an ultrahigh areal capacity of 1000 mAh cm-2 (volumetric capacity of ≈6000 mAh cm-3 ), and a Coulombic efficiency of 99.4% on a carbon substrate, surpassing the state-of-the-art metal electrodes by approximately two orders of magnitude, are realized. Furthermore, as a proof-of-concept, a series of full cells based on the Ni anode is developed. The designed Ni-MnO2 full battery exhibits a long lifespan of 2000 cycles, while the Ni-PbO2 full battery achieves a high areal capacity of 200 mAh cm-2 . The findings of this study are important for enlightening a new arena toward the advancement of dendrite-free Ni-metal anodes with ultrahigh capacities and long cycle life for various energy-storage devices
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|a Journal Article
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|a Ni anodes
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|a Ni-metal batteries
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|a electrolyte regulation
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|a metal electroplating/stripping
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| 650 |
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4 |
|a ultrahigh capacities
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1 |
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|a Meng, Yahan
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Gao, Pengfei
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Li, Ke
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Liu, Zaichun
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Zhu, Zhengxin
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Ali, Mohsin
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Ahmad, Touqeer
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Chen, Na
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Yuan, Yuan
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Xu, Yan
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Chuai, Mingyan
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Sun, Jifei
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Zheng, Xinhua
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Li, Xingxing
|e verfasserin
|4 aut
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| 700 |
1 |
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|a Yang, Jinlong
|e verfasserin
|4 aut
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| 700 |
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|a Chen, Wei
|e verfasserin
|4 aut
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| 773 |
0 |
8 |
|i Enthalten in
|t Advanced materials (Deerfield Beach, Fla.)
|d 1998
|g 35(2023), 42 vom: 17. Okt., Seite e2305368
|w (DE-627)NLM098206397
|x 1521-4095
|7 nnns
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| 773 |
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|g volume:35
|g year:2023
|g number:42
|g day:17
|g month:10
|g pages:e2305368
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|u http://dx.doi.org/10.1002/adma.202305368
|3 Volltext
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